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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Pireaux, Jean Jacques
University of Namur
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (12/12 displayed)
- 2023Plasma Treatment of Polystyrene Films—Effect on Wettability and Surface Interactions with Au Nanoparticlescitations
- 2022Low-pressure plasma process for the dry synthesis of cactus-like Au-TiO2 nanocatalysts for toluene degradationcitations
- 2022X-ray Photoelectron Spectroscopy (XPS) Analysis of Ultrafine Au Nanoparticles Supported over Reactively Sputtered TiO 2 Filmscitations
- 2022Low-pressure plasma process for the dry synthesis of cactus-like Au-TiO 2 nanocatalysts for toluene degradationcitations
- 2021Compositional, structural, morphological, and optical properties of ZnO thin films prepared by PECVD techniquecitations
- 2020Using ammonia for reactive magnetron sputtering, a possible alternative to HiPIMS?citations
- 2020Formable chromium nitride coatings for proton exchange membrane fuel cell stainless steel bipolar platescitations
- 2019Carbon-based lanthanum nickelate material La 2−x−y Nd x Pr y NiO 4+δ (x = 0, 0.3, and 0.5; y = 0 and 0.2) as a bifunctional electrocatalyst for oxygen reduction in alkaline mediacitations
- 2019Defective Pt–Ni/graphene nanomaterials by simultaneous or sequential treatments of organometallic precursors by low-pressure oxygen plasmacitations
- 2018Wide range investigation of duty cycle and frequency effects on bipolar magnetron sputtering of chromium nitridecitations
- 2015Interface and Composition Analysis on Perovskite Solar Cellscitations
- 2015Air-stable, non-volatile resistive memory based on hybrid organic/inorganic nanocompositescitations
Places of action
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article
Low-pressure plasma process for the dry synthesis of cactus-like Au-TiO2 nanocatalysts for toluene degradation
Abstract
<p>The development of environment-friendly, low-cost and efficient catalyst preparation processes has always been a major issue in the field of catalysis. Wet chemistry methods are often used but these techniques are not sustainable, as post waste solution treatment remains an important drawback. Here an innovative dry low-pressure plasma process for metal nanoparticles supported nanocatalysts preparation is reported. The solid metal and oxide support precursors are physically mixed and then exposed to a radiofrequency Ar/N<sub>2</sub> plasma discharge, leading to the precursor degradation and the subsequent nanoparticles generation, without pre- or post- preparation steps. The metal nanoparticle loading and the particle size of metal and oxide support can be easily tuned by changing the ratio of the precursor materials, making the process simple, versatile, highly efficient, and scalable. As a proof of concept, gold nanoparticles (Au NPs) supported on titanium dioxide (TiO<sub>2</sub>) were prepared and tested as nanocatalysts for toluene (C<sub>7</sub>H<sub>8</sub>) degradation at temperatures ranging from 25 to 450 °C. Up to 100% of C<sub>7</sub>H<sub>8</sub> conversion into CO<sub>2</sub> was achieved over the Au-TiO<sub>2</sub> nanocatalysts, demonstrating that this dry method is a very efficient way to prepare highly active nanocatalysts.</p>