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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Douthwaite, Richard E.
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (11/11 displayed)
- 2021Hierarchical bismuth vanadate/reduced graphene oxide composite photocatalyst for hydrogen evolution and bisphenol A degradationcitations
- 2020Pompon Dahlia-like Cu2O/rGO Nanostructures for Visible Light Photocatalytic H2 Production and 4-Chlorophenol Degradationcitations
- 2020Pompon Dahlia‐like Cu2O/rGO Nanostructures for Visible Light Photocatalytic H2 Production and 4‐Chlorophenol Degradationcitations
- 2018Delaminated CoAl-Layered Double Hydroxide@TiO2Heterojunction Nanocomposites for Photocatalytic Reduction of CO2citations
- 2018Delaminated CoAl‐Layered Double Hydroxide@TiO2 Heterojunction Nanocomposites for Photocatalytic Reduction of CO2citations
- 2018Delaminated CoAl-Layered Double Hydroxide@TiO2 Heterojunction Nanocomposites for CO2 Photocatalytic Reduction
- 2017P25@CoAl layered double hydroxide heterojunction nanocomposites for CO 2 photocatalytic reductioncitations
- 2017P25@CoAl layered double hydroxide heterojunction nanocomposites for CO2 photocatalytic reduction
- 2017P25@CoAl layered double hydroxide heterojunction nanocomposites for CO2 photocatalytic reductioncitations
- 2017Delaminated CoAl-Layered Double Hydroxide at TiO2 Heterojunction Nanocomposites for Photocatalytic Reduction of CO2citations
- 2009Synthesis, Coordination Chemistry and Bonding of Strong N-Donor Ligands Incorporating the 1H-Pyridin-(2E)-Ylidene (PYE) Motifcitations
Places of action
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article
P25@CoAl layered double hydroxide heterojunction nanocomposites for CO2 photocatalytic reduction
Abstract
Artificial photosynthesis driven by inorganic photocatalysts offers a promising route to renewable solar fuels, however efficient CO2 photoreduction remains a challenge. A family of hierarchical nanocomposites, comprising P25 nanoparticles encapsulated within microporous CoAl-layered double hydroxides (CoAl-LDHs) were prepared via a one-pot hydrothermal synthesis. Heterojunction formation between the visible light absorbing CoAl-LDH and UV light absorbing P25 semiconductors extends utilisation of the solar spectrum, while the solid basicity of the CoAl-LDH increases CO2 availability at photocatalytic surfaces. Matching of the semiconductor band structures and strong donor–acceptor coupling improves photoinduced charge carrier separation and transfer via the heterojunction. Hierarchical P25@CoAl-LDH nanocomposites exhibit good activity and selectivity (>90%) for aqueous CO2 photoreduction to CO, without a sacrificial hole acceptor. This represents a facile and cost-effective strategy for the design and development of LDH-based nanomaterials for efficient photocatalysis for renewable solar fuel production from particularly CO2 and water.