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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Bund, Andreas
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (23/23 displayed)
- 2024A Novel Method for Preparation of Al–Ni Reactive Coatings by Incorporation of Ni Nanoparticles into an Al Matrix Fabricated by Electrodeposition in AlCl<sub>3</sub>:1‐Eethyl‐3‐Methylimidazolium Chloride (1.5:1) Ionic Liquid Containing Ni Nanoparticles
- 2024Integration of Multijunction Absorbers and Catalysts for Efficient Solar‐Driven Artificial Leaf Structures: A Physical and Materials Science Perspectivecitations
- 2023Analysis of Pre-Treatment Processes to Enable Electroplating on Nitrided Steel
- 2023Electrochemical reduction of tantalum and titanium halides in 1-butyl-1-methylpyrrolidinium bis (trifluoromethyl-sulfonyl)imide and 1-butyl-1-methylpyrrolidinium trifluoromethanesulfonate ionic liquids
- 2023Quasi-in-Situ Analysis of Electropolished Additively Manufactured Stainless Steel Surfaces
- 2022Hollow platinum-gold and palladium-gold nanoparticles: synthesis and characterization of composition-structure relationshipcitations
- 2022Corrosion Properties of Ni-P-B Dispersion Coating for Industrial Knives and Bladescitations
- 2022Selective Metallization of Polymers: Surface Activation of Polybutylene Terephthalate (PBT) Assisted by Picosecond Laser Pulsescitations
- 2021Selective metallization of polymers: surface activation of polybutylene terephthalate (PBT) assisted by picosecond laser pulsescitations
- 2021The need for digitalisation in electroplating – How digital approaches can help to optimize the electrodeposition of chromium from trivalent electrolytes
- 2021Anti-corrosive siloxane coatings for improved long-term performance of supercapacitors with an aqueous electrolytecitations
- 2021Analysis of the physical and photoelectrochemical properties of c-Si(p)/a-SiC:H(p) photocathodes for solar water splittingcitations
- 2020Aluminium-poly(3,4-ethylenedioxythiophene) rechargeable battery with ionic liquid electrolytecitations
- 2019Relation between color and surface morphology of electrodeposited chromium for decorative applicationscitations
- 2019Fluidic self-assembly on electroplated multilayer solder bumps with tailored transformation imprinted melting pointscitations
- 2019Electrochemical deposition of silicon from a sulfolane-based electrolyte: effect of applied potentialcitations
- 2019Nanoscale morphological changes at lithium interface, triggered by the electrolyte composition and electrochemical cyclingcitations
- 2018Structure and formation of trivalent chromium conversion coatings containing cobalt on zinc plated steelcitations
- 2017An electrochemical quartz crystal microbalance study on electrodeposition of aluminum and aluminum-manganese alloyscitations
- 2016Ultrasound assisted electrodeposition of Zn and Zn-TiO2 coatingscitations
- 2012Electrochemical supercapacitors based on a novel graphene/conjugated polymer composite systemcitations
- 2010Do solvation layers of ionic liquids influence electrochemical reactions?citations
- 2009Novel amino-acid-based polymer/multi-walled carbon nanotube bio-nanocompositescitations
Places of action
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article
Integration of Multijunction Absorbers and Catalysts for Efficient Solar‐Driven Artificial Leaf Structures: A Physical and Materials Science Perspective
Abstract
<jats:p> Artificial leaves could be the breakthrough technology to overcome the limitations of storage and mobility through the synthesis of chemical fuels from sunlight, which will be an essential component of a sustainable future energy system. However, the realization of efficient solar‐driven artificial leaf structures requires integrated specialized materials such as semiconductor absorbers, catalysts, interfacial passivation, and contact layers. To date, no competitive system has emerged due to a lack of scientific understanding, knowledge‐based design rules, and scalable engineering strategies. Herein, competitive artificial leaf devices for water splitting, focusing on multiabsorber structures to achieve solar‐to‐hydrogen conversion efficiencies exceeding 15%, are discussed. A key challenge is integrating photovoltaic and electrochemical functionalities in a single device. Additionally, optimal electrocatalysts for intermittent operation at photocurrent densities of 10–20 mA cm<jats:sup>−2</jats:sup> must be immobilized on the absorbers with specifically designed interfacial passivation and contact layers, so‐called buried junctions. This minimizes voltage and current losses and prevents corrosive side reactions. Key challenges include understanding elementary steps, identifying suitable materials, and developing synthesis and processing techniques for all integrated components. This is crucial for efficient, robust, and scalable devices. Herein, corresponding research efforts to produce green hydrogen with unassisted solar‐driven (photo‐)electrochemical devices are discussed and reported.</jats:p>