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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Wang, Dong
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (17/17 displayed)
- 2024Engineered Anchor Peptide LCI with a Cobalt Cofactor Enhances Oxidation Efficiency of Polystyrene Microparticlescitations
- 2024Hydrogen diffusivity in X65 pipeline steel: Desorption and permeation studiescitations
- 2024Low-temperature process design for inversion mode n-channel thin-film-transistor on polycrystalline Ge formed by solid-phase crystallizationcitations
- 2024Controllable Si oxidation mediated by annealing temperature and atmosphere
- 2024Safe pipelines for hydrogen transportcitations
- 2024Integration of Multijunction Absorbers and Catalysts for Efficient Solar‐Driven Artificial Leaf Structures: A Physical and Materials Science Perspectivecitations
- 2023Gold nanosponges: fascinating optical properties of a unique disorder-dominated systemcitations
- 2022A dual functional chondro-inductive chitosan thermogel with high shear modulus and sustained drug release for cartilage tissue engineeringcitations
- 2022Controllable Si oxidation mediated by annealing temperature and atmospherecitations
- 2022Thin film nanostructuring at oblique angles by substrate patterning
- 2021Rapid fabrication and interface structure of highly faceted epitaxial Ni-Au solid solution nanoparticles on sapphirecitations
- 2019Investigation of a surface mounted pm machine concept with 3d-flux paths, modular stator and amorphous materialcitations
- 2018The effect of in-situ hydrogen plasma charging on the hydrogen embrittlement susceptibility of DP and TRIP steel
- 2016Solid-state dewetting of single- and bilayer Au-W thin films: unraveling the role of individual layer thickness, stacking sequence and oxidation on morphology evolutioncitations
- 2014A highly active and magnetically recoverable tris(triazolyl)-CuI catalyst for alkyne-azide cycloaddition reactionscitations
- 2013Nuclear resonance vibrational spectroscopic and computational study of high-valent diiron complexes relevant to enzyme intermediates.citations
- 2005Polymerization and carbonization of high internal phase emulsionscitations
Places of action
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article
Integration of Multijunction Absorbers and Catalysts for Efficient Solar‐Driven Artificial Leaf Structures: A Physical and Materials Science Perspective
Abstract
<jats:p> Artificial leaves could be the breakthrough technology to overcome the limitations of storage and mobility through the synthesis of chemical fuels from sunlight, which will be an essential component of a sustainable future energy system. However, the realization of efficient solar‐driven artificial leaf structures requires integrated specialized materials such as semiconductor absorbers, catalysts, interfacial passivation, and contact layers. To date, no competitive system has emerged due to a lack of scientific understanding, knowledge‐based design rules, and scalable engineering strategies. Herein, competitive artificial leaf devices for water splitting, focusing on multiabsorber structures to achieve solar‐to‐hydrogen conversion efficiencies exceeding 15%, are discussed. A key challenge is integrating photovoltaic and electrochemical functionalities in a single device. Additionally, optimal electrocatalysts for intermittent operation at photocurrent densities of 10–20 mA cm<jats:sup>−2</jats:sup> must be immobilized on the absorbers with specifically designed interfacial passivation and contact layers, so‐called buried junctions. This minimizes voltage and current losses and prevents corrosive side reactions. Key challenges include understanding elementary steps, identifying suitable materials, and developing synthesis and processing techniques for all integrated components. This is crucial for efficient, robust, and scalable devices. Herein, corresponding research efforts to produce green hydrogen with unassisted solar‐driven (photo‐)electrochemical devices are discussed and reported.</jats:p>