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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Moser, Maximilian
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (12/12 displayed)
- 2024The Role Of Side Chains and Hydration on Mixed Charge Transport in N-Type Polymer Films.citations
- 2023Role of aggregates and microstructure of mixed-ionic-electronic-conductors on charge transport in electrochemical transistors.citations
- 2022Infrared Organic Photodetectors Employing Ultralow Bandgap Polymer and Non‐Fullerene Acceptors for Biometric Monitoringcitations
- 2022Oligoethylene Glycol Side Chains Increase Charge Generation in Organic Semiconductor Nanoparticles for Enhanced Photocatalytic Hydrogen Evolutioncitations
- 2022Synthetic nuances to maximize n-type organic electrochemical transistor and thermoelectric performance in fused lactam polymerscitations
- 2022Synthetic Nuances to Maximize n-Type Organic Electrochemical Transistor and Thermoelectric Performance in Fused Lactam Polymers.citations
- 2022The effect of glycol side chains on the assembly and microstructure of conjugated polymerscitations
- 2021Ternary organic photodetectors based on pseudo-binaries nonfullerene-based acceptorscitations
- 2021Regiochemistry-driven organic electrochemical transistor performance enhancement in ethylene glycol-functionalized polythiophenescitations
- 2020Side Chain Redistribution as a Strategy to Boost Organic Electrochemical Transistor Performance and Stabilitycitations
- 2020Side Chain Redistribution as a Strategy to Boost Organic Electrochemical Transistor Performance and Stability.citations
- 2019Reversible Electronic Solid-Gel Switching of a Conjugated Polymercitations
Places of action
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article
Infrared Organic Photodetectors Employing Ultralow Bandgap Polymer and Non‐Fullerene Acceptors for Biometric Monitoring
Abstract
<jats:title>Abstract</jats:title><jats:p>Recent efforts in the field of organic photodetectors (OPD) have been focused on extending broadband detection into the near‐infrared (NIR) region. Here, two blends of an ultralow bandgap push–pull polymer TQ‐T combined with state‐of‐the‐art non‐fullerene acceptors, IEICO‐4F and Y6, are compared to obtain OPDs for sensing in the NIR beyond 1100 nm, which is the cut off for benchmark Si photodiodes. It is observed that the TQ‐T:IEICO‐4F device has a superior IR responsivity (0.03 AW<jats:sup>‐1</jats:sup> at 1200 nm and −2 V bias) and can detect infrared light up to 1800 nm, while the TQ‐T:Y6 blend shows a lower responsivity of 0.01 AW<jats:sup>‐1</jats:sup>. Device physics analyses are tied with spectroscopic and morphological studies to link the superior performance of TQ‐T:IEICO‐4F OPD to its faster charge separation as well as more favorable donor–acceptor domains mixing. In the polymer blend with Y6, the formation of large agglomerates that exceed the exciton diffusion length, which leads to high charge recombination, is observed. An application of these devices as biometric sensors for real‐time heart rate monitoring via photoplethysmography, utilizing infrared light, is demonstrated.</jats:p>