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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Gasparini, Nicola
Imperial College London
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (20/20 displayed)
- 2024Dark Current in Broadband Perovskite–Organic Heterojunction Photodetectors Controlled by Interfacial Energy Band Offsetcitations
- 2024A novel selenophene based non-fullerene acceptor for near-infrared organic photodetectors with ultra-low dark currentcitations
- 2023Semitransparent Organic Photovoltaics Utilizing Intrinsic Charge Generation in Non‐Fullerene Acceptorscitations
- 2023Enhanced sub-1 eV detection in organic photodetectors through tuning polymer energetics and microstructurecitations
- 2023Neuromorphic computing based on halide perovskitescitations
- 2022Infrared Organic Photodetectors Employing Ultralow Bandgap Polymer and Non‐Fullerene Acceptors for Biometric Monitoringcitations
- 2022Synthetic nuances to maximize n-type organic electrochemical transistor and thermoelectric performance in fused lactam polymerscitations
- 2022Correlating Acceptor Structure and Blend Nanostructure with the Photostability of Nonfullerene Organic Solar Cellscitations
- 2022Synthetic Nuances to Maximize n-Type Organic Electrochemical Transistor and Thermoelectric Performance in Fused Lactam Polymers.citations
- 2022Overcoming nanoscale inhomogeneities in thin-film perovskites via exceptional post-annealing grain growth for enhanced photodetectioncitations
- 2021Interface Molecular engineering for laminated monolithic perovskite/silicon tandem solar cells with 80.4% fill factorcitations
- 2021Ternary organic photodetectors based on pseudo-binaries nonfullerene-based acceptorscitations
- 2020Side Chain Redistribution as a Strategy to Boost Organic Electrochemical Transistor Performance and Stabilitycitations
- 2020Side Chain Redistribution as a Strategy to Boost Organic Electrochemical Transistor Performance and Stability.citations
- 2020Unraveling the Complex Nanomorphology of Ternary Organic Solar Cells with Multimodal Analytical Transmission Electron Microscopycitations
- 2019Favorable Mixing Thermodynamics in Ternary Polymer Blends for Realizing High Efficiency Plastic Solar Cellscitations
- 2017Indacenodithienothiophene-Based Ternary Organic Solar Cellscitations
- 2017Controlling charge carrier recombination in ternary organic solar cells ; Unterdrückung von Ladungsträgerrekombination in ternären organischen Solarzellen
- 2016A Series of Pyrene-Substituted Silicon Phthalocyanines as Near-IR Sensitizers in Organic Ternary Solar Cellscitations
- 2015Integrated Molecular, Morphological and Interfacial Engineering towards Highly Efficient and Stable Solution-processed Small Molecule Organic Solar Cellscitations
Places of action
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article
Infrared Organic Photodetectors Employing Ultralow Bandgap Polymer and Non‐Fullerene Acceptors for Biometric Monitoring
Abstract
<jats:title>Abstract</jats:title><jats:p>Recent efforts in the field of organic photodetectors (OPD) have been focused on extending broadband detection into the near‐infrared (NIR) region. Here, two blends of an ultralow bandgap push–pull polymer TQ‐T combined with state‐of‐the‐art non‐fullerene acceptors, IEICO‐4F and Y6, are compared to obtain OPDs for sensing in the NIR beyond 1100 nm, which is the cut off for benchmark Si photodiodes. It is observed that the TQ‐T:IEICO‐4F device has a superior IR responsivity (0.03 AW<jats:sup>‐1</jats:sup> at 1200 nm and −2 V bias) and can detect infrared light up to 1800 nm, while the TQ‐T:Y6 blend shows a lower responsivity of 0.01 AW<jats:sup>‐1</jats:sup>. Device physics analyses are tied with spectroscopic and morphological studies to link the superior performance of TQ‐T:IEICO‐4F OPD to its faster charge separation as well as more favorable donor–acceptor domains mixing. In the polymer blend with Y6, the formation of large agglomerates that exceed the exciton diffusion length, which leads to high charge recombination, is observed. An application of these devices as biometric sensors for real‐time heart rate monitoring via photoplethysmography, utilizing infrared light, is demonstrated.</jats:p>