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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Douthwaite, Richard E.
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (11/11 displayed)
- 2021Hierarchical bismuth vanadate/reduced graphene oxide composite photocatalyst for hydrogen evolution and bisphenol A degradationcitations
- 2020Pompon Dahlia-like Cu2O/rGO Nanostructures for Visible Light Photocatalytic H2 Production and 4-Chlorophenol Degradationcitations
- 2020Pompon Dahlia‐like Cu2O/rGO Nanostructures for Visible Light Photocatalytic H2 Production and 4‐Chlorophenol Degradationcitations
- 2018Delaminated CoAl-Layered Double Hydroxide@TiO2Heterojunction Nanocomposites for Photocatalytic Reduction of CO2citations
- 2018Delaminated CoAl‐Layered Double Hydroxide@TiO2 Heterojunction Nanocomposites for Photocatalytic Reduction of CO2citations
- 2018Delaminated CoAl-Layered Double Hydroxide@TiO2 Heterojunction Nanocomposites for CO2 Photocatalytic Reduction
- 2017P25@CoAl layered double hydroxide heterojunction nanocomposites for CO 2 photocatalytic reductioncitations
- 2017P25@CoAl layered double hydroxide heterojunction nanocomposites for CO2 photocatalytic reduction
- 2017P25@CoAl layered double hydroxide heterojunction nanocomposites for CO2 photocatalytic reductioncitations
- 2017Delaminated CoAl-Layered Double Hydroxide at TiO2 Heterojunction Nanocomposites for Photocatalytic Reduction of CO2citations
- 2009Synthesis, Coordination Chemistry and Bonding of Strong N-Donor Ligands Incorporating the 1H-Pyridin-(2E)-Ylidene (PYE) Motifcitations
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article
Delaminated CoAl‐Layered Double Hydroxide@TiO2 Heterojunction Nanocomposites for Photocatalytic Reduction of CO2
Abstract
<jats:title>Abstract</jats:title><jats:p>Photocatalytic reduction offers an attractive route for CO<jats:sub>2</jats:sub> utilization as a chemical feedstock for solar fuels production but remains challenging due to the poor efficiency, instability, and/or toxicity of current catalyst systems. Delaminated CoAl‐layered double hydroxide nanosheets (LDH‐DS) combined with TiO<jats:sub>2</jats:sub> nanotubes (NTs) or nanoparticles (NPs) are promising nanocomposite photocatalysts for CO<jats:sub>2</jats:sub> reduction. Heterojunction formation between visible light absorbing delaminated CoAl nanosheets and UV light absorbing TiO<jats:sub>2</jats:sub> nanotubes greatly enhances interfacial contact between both high aspect ratio components relative to their bulk counterparts. The resulting synergic interaction confers a significant improvement in photoinduced charge carrier separation, and concomitant aqueous phase CO<jats:sub>2</jats:sub> photocatalytic reduction, in the absence of a sacrificial hole acceptor. CO productivity for a 3 wt% LDH‐DS@TiO<jats:sub>2</jats:sub>‐NT nanocomposite of 4.57 µmol g<jats:sub>cat</jats:sub><jats:sup>‐1</jats:sup> h<jats:sup>‐1</jats:sup> exhibits a tenfold and fivefold increase over that obtained for individual TiO<jats:sub>2</jats:sub> NT and delaminated CoAl‐LDH components respectively and is double that obtained for 3 wt% bulk‐LDH@TiO<jats:sub>2</jats:sub>‐NT and 3 wt% LDH‐DS@TiO<jats:sub>2</jats:sub>‐NP catalysts. Synthesis of delaminated LDH and metal oxide nanocomposites represents a cost‐effective strategy for aqueous phase CO<jats:sub>2</jats:sub> reduction.</jats:p>