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Tzourtzouklis, Ioannis
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article
Supersoft Polymer Melts in Binary Blends of Bottlebrush cis‐1,4‐Polyfarnesene and cis‐1,4‐Polyisoprene
Abstract
<jats:title>Abstract</jats:title><jats:p>Binary blends of polyterpenes are employed comprising <jats:italic>cis</jats:italic>‐1,4‐polyfarnesene (PF) with a bottlebrush architecture, and linear <jats:italic>cis</jats:italic>‐1,4‐polyisoprene (PI) as model systems toward supersoft polymer melts. The bottlebrush PF results in a low plateau modulus ( Pa) that can further be reduced with the addition of PI. Depending on the fraction of short PI chains in the <jats:italic>athermal</jats:italic> and nearly <jats:italic>isofrictional</jats:italic> blends, plateau moduli in the range from 1 to 10 kPa can be achieved. Tube dilation is very efficient in the present binary blends as compared to more common blends comprising long/short or linear/star chains of identical polymer structure.</jats:p>