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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Wang, Xianbao
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article
2D MXenes Embedded Perovskite Hydrogels for Efficient and Stable Solar Evaporation
Abstract
<jats:title>Abstract</jats:title><jats:p>Solar evaporation is a facile and promising technology to efficiently utilize renewable energy for freshwater production and seawater desalination. Here, the fabrication of self‐regenerating hydrogel composed of 2D‐MXenes nanosheets embedded in perovskite La <jats:sub>0.6</jats:sub>Sr <jats:sub>0.4</jats:sub>Co <jats:sub>0.2</jats:sub>Fe <jats:sub>0.8</jats:sub>O<jats:sub>3−</jats:sub><jats:italic><jats:sub>δ</jats:sub></jats:italic> (LSCF)/polyvinyl alcohol hydrogels for efficient solar‐driven evaporation and seawater desalination is reported. The mixed dimensional LSCF/Ti<jats:sub>3</jats:sub>C<jats:sub>2</jats:sub> composite features a localized surface plasmonic resonance effect in the polymeric network of polyvinyl alcohol endows excellent evaporation rates (1.98 kg m<jats:sup>−2</jats:sup> h<jats:sup>−1</jats:sup>) under 1 k Wm<jats:sup>−2</jats:sup> or one sun solar irradiation ascribed by hydrophilicity and broadband solar absorption (96%). Furthermore, the long‐term performance reveals smooth mass change (13.33 kg m<jats:sup>−2</jats:sup>) during 8 h under one sun. The composite hydrogel prompts the dilution of concentrated brines and redissolves it back to water (1.2 g NaCl/270 min) without impeding the evaporation rate without any salt‐accumulation. The present research offers a substantial opportunity for solar‐driven evaporation without any salt accumulation in real‐life applications.</jats:p>