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Cabrita, Luis
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article
Membranes with a low loading of Metal–Organic Framework-Supported Ionic Liquids for CO2/N2 separation in CO2 capture
Abstract
<p>Immobilization of ionic liquids (ILs) into 3D metal–organic frameworks (MOFs) is reported. The incorporation of these composites in a polyimide-based matrix (Matrimid® 5218) to yield [IL@MOF]@Matrimid® 5218 is an efficient strategy to improve the permeability and selectivity toward CO<sub>2</sub>/N<sub>2</sub> mixtures, presenting also a remarkable improvement in membrane flexibility and mechanical resistance. Using MOF-5, a crystalline phase different to its original phase is obtained after the incorporation of hydrated IL without loss of adsorptive properties.</p>