693.932 PEOPLE
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| Naji, M. |
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Auban-Senzier, Pascale
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Topics
Publications (32/32 displayed)
- 2024A highly conducting tetrathiafulvalene-tetracarboxylate based dysprosium(iii) 2D metal-organic framework with single molecule magnet behaviourcitations
- 2023Bis(Vinylenedithio)‐Tetrathiafulvalene‐Based Coordination Networkscitations
- 2022Bis(Vinylenedithio)-Tetrathiafulvalene-Based Coordination Networkscitations
- 2021Old Donors for New Molecular Conductors: Combining TMTSF and BEDT-TTF with Anionic (TaF6)1−x/(PF6)x Alloyscitations
- 2020Chiral Conducting Me-EDT-TTF and Et-EDT-TTFBased Radical Cation Salts with the Perchlorate Anion
- 2020Combining Chirality and Hydrogen Bonding in Methylated Ethylenedithio-Tetrathiafulvalene Primary Diamide Precursors and Radical Cation Saltscitations
- 2020Conservation of structural arrangements and 3 : 1 stoichiometry in a series of crystalline conductors of TMTTF, TMTSF, BEDT-TTF, and chiral DM-EDT-TTF with the oxo-bis[pentafluorotantalate( v )] dianioncitations
- 2020Chiral Conducting Me-EDT-TTF and Et-EDT-TTF-Based Radical Cation Salts with the Perchlorate Anioncitations
- 2020Glycine Residue Twists HOMO···HOMO Interactions in a Molecular Conductor
- 2020Glycine Residue Twists HOMO…HOMO Interactions in a Molecular Conductorcitations
- 2020In Search of Chiral Molecular Superconductors: κ‐[( S,S )‐DM‐BEDT‐TTF] 2 ClO 4 Revisitedcitations
- 2020Conservation of structural arrangements and 3 : 1 stoichiometry in a series of crystalline conductors of TMTTF, TMTSF, BEDT-TTF, and chiral DM-EDTTTF with the oxo-bis[pentafluorotantalate(V)] dianion
- 2019Chiral EDT-TTF precursors with one stereogenic centre: substituent size modulation of the conducting properties in the (R-EDT-TTF)2PF6 (R = Me or Et) series
- 2019Chiral EDT-TTF precursors with one stereogenic centre: substituent size modulation of the conducting properties in the (R-EDT-TTF) 2 PF 6 (R = Me or Et) seriescitations
- 2018Conducting Anilate-Based Mixed-Valence Fe(II)Fe(III) Coordination Polymer: Small-Polaron Hopping Model for Oxalate-Type Fe(II)Fe(III) 2D Networkscitations
- 2018Conducting Anilate-Based Mixed-Valence Fe(II)Fe(III) Coordination Polymer: Small-Polaron Hopping Model for Oxalate-Type Fe(II)Fe(III) 2D Networks
- 2018Influence of carrier lifetime on quantum criticality and superconducting T c of (TMTSF) 2 ClO 4
- 2017Synthesis and Physical Properties of Purely Organic BEDT-TTF-Based Conductors Containing Hetero-/Homosubstituted Cl/CN-Anilate Derivativescitations
- 2017Synthesis and physical properties of purely organic BEDT-TTF-based conductors containing hetero-/homosubstituted Cl/CN-anilate derivativescitations
- 2016Localization versus delocalization in chiral single component conductors of gold bis(dithiolene) complexescitations
- 2015Metal-charge density wave coexistence in TTF[Ni(dmit)2]2
- 2014Structural Diversity and Physical Properties of Paramagnetic Molecular Conductors Based on Bis(ethylenedithio)tetrathiafulvalene (BEDT-TTF) and the Tris(chloranilato)ferrate(III) Complexcitations
- 2014Electrical magnetochiral anisotropy in a bulk chiral molecular conductorcitations
- 2013Chirality Driven Metallic versus Semiconducting Behavior in a Complete Series of Radical Cation Salts Based on Dimethyl-Ethylenedithio-Tetrathiafulvalene (DM-EDT-TTF)citations
- 2012Anisotropic chemical pressure effects in single-component molecular metals based on radical dithiolene and diselenolene gold complexes.citations
- 2011Dual proton / hole mixed valence in a molecular metal: balancing chemical activity in the solid state by tapping into a molecular hole reservoircitations
- 2010Order versus disorder in chiral tetrathiafulvalene-oxazoline radical-cation salts: structural and theoretical investigations and physical properties.citations
- 2010Linear-T scattering and pairing from antiferromagnetic fluctuations in the (TMTSF)_2X organic superconductorscitations
- 2009Domain walls at the spin density wave endpoint of the organic superconductor (TMTSF)2PF6 under pressure
- 2009A Single-Component Molecular Metal Based on a Thiazole Dithiolate Gold Complexcitations
- 2008A series of strongly one-dimensional organic metals with strictly uniform stacks: (o-DMTTF)2X (X = Cl, Br, I)citations
- 2004Suppression of superconductivity by non-magnetic disorder in the organic superconductor (TMTSF)2(ClO4)(1-x)(ReO4)x.citations
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article
Bis(Vinylenedithio)‐Tetrathiafulvalene‐Based Coordination Networks
Abstract
International audience ; Novel coordination polymers embedding electroactive moieties present a high interest in the development of porous conducting materials. While tetrathiafulvalene (TTF) based metal-organic frameworks were reported to yield through-space conducting frameworks, the use of S-enriched scaffolds remains elusive in this field. Herein is reported the employment of bis(vinylenedithio)tetrathiafulvalene (BVDT-TTF) functionalized with pyridine coordinating moieties in coordination polymers. Its combination with various transition metals yielded four isostructural networks, whose conductivity increased upon chemical oxidation with iodine. The oxidation was confirmed in a singlecrystal to single-crystal X-ray diffraction experiment for the Cd(II) complex. Raman spectroscopy measurements and DFT calculations confirmed the oxidation state of the bulk materials, and band structure calculations assessed the ground state as an electronically localized antiferromagnetic state, while the conduction occurs in a 2D manner. These results are shedding light to comprehend how to improve through-space conductivity thanks to sulfur enriched ligands.