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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Danner, Timo
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (13/13 displayed)
- 2024Lithium Redistribution Mechanism within Silicon-Graphite Electrodes: Multi-Method Approach and Method Validationcitations
- 2024Influence of Electrode Structuring Techniques on the Performance of All‐Solid‐State Batteriescitations
- 2024Lithiophilic interlayer driven 'bottom-up' metal infilling in high current density Li-metal anodescitations
- 2024Strategies to Spatially Guide Li Deposition in Porous Electrodes for High-Performance Lithium Metal Batteries
- 2024Synergistic Enhancement of Mechanical and Electrochemical Properties in Grafted Polymer/Oxide Hybrid Electrolytescitations
- 2024Material parameters affecting Li plating in Si/graphite composite electrodescitations
- 2023Effect of Particle Size and Pressure on the Transport Properties of the Fast Ion Conductor t-Li7SiPS8citations
- 2023Optimizing the Composite Cathode Microstructure in All‐Solid‐State Batteries by Structure‐Resolved Simulations
- 2022Effect of Particle Size and Pressure on the Transport Properties of the Fast Ion Conductor t-Li7SiPS8
- 2020Investigating the Nucleation of Lithium Deposits in Polycrystalline Solid Electrolytes
- 2020Mechanistic details of the spontaneous intercalation of Li metal into graphite electrodem
- 2019The importance of passive materials in Li-Ion battery electrodes
- 2012A Flexible Framework for Modeling Multiple Solid, Liquid and Gaseous Phases in Batteries and Fuel Cellscitations
Places of action
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article
Influence of Electrode Structuring Techniques on the Performance of All‐Solid‐State Batteries
Abstract
All-solid-state batteries (ASSBs) offer a promising route to safer batteries with superior energy density compared to conventional Li-ion batteries (LIBs). However, the design of the composite cathode and optimization of the underlying microstructure is one of the aspects requiring intensive research. Achieving both high energy and power density remains challenging due to limitations in ionic conductivity and active material loading. Using structure-resolved simulations, we investigate the potential of perforated and layered electrode designs to enhance ASSB performance. Design strategies showing significant performance increase in LIBs are evaluated regarding their application to ASSBs. Composite cathodes with solid electrolyte channels in the structure do not significantly increase cell performance compared to unstructured electrodes. However, the design with a two-layer cathode proves promising. The layered structure effectively balances improved ionic transport due to increased solid electrolyte fraction at the separator side and substantial active material loading through increased active material fraction at the current collector side of the cathode. Our research highlights key challenges in ASSB development and provides a clear direction for future studies in the field.