Materials Map

Discover the materials research landscape. Find experts, partners, networks.

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The Materials Map is an open tool for improving networking and interdisciplinary exchange within materials research. It enables cross-database search for cooperation and network partners and discovering of the research landscape.

The dashboard provides detailed information about the selected scientist, e.g. publications. The dashboard can be filtered and shows the relationship to co-authors in different diagrams. In addition, a link is provided to find contact information.

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The Materials Map is still under development. In its current state, it is only based on one single data source and, thus, incomplete and contains duplicates. We are working on incorporating new open data sources like ORCID to improve the quality and the timeliness of our data. We will update Materials Map as soon as possible and kindly ask for your patience.

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in Cooperation with on an Cooperation-Score of 37%

Topics

Publications (3/3 displayed)

  • 2021Tricyanidoferrates(−IV) and Ruthenates(−IV) with Non-Innocent Cyanido Ligands7citations
  • 2021Valence fluctuations in the 3D + 3 modulated Yb3Co4Ge13 Remeika phase9citations
  • 2018BiMn: Synthesis, separation by centrifugation, and characterization16citations

Places of action

Chart of shared publication
Eng, Lukas
1 / 26 shared
Amber, Zeeshan H.
1 / 1 shared
Kaiser, Martin
1 / 7 shared
Prots, Yurii
1 / 5 shared
Höhn, Peter
1 / 2 shared
Jesche, Anton
1 / 4 shared
Hunger, Jens
1 / 4 shared
Rüsing, Michael
1 / 2 shared
Jach, Franziska
1 / 1 shared
Ruck, Michael
1 / 74 shared
Wagner, Frank R.
1 / 1 shared
Wagler, Jörg
1 / 3 shared
Feig, Manuel
1 / 1 shared
Motylenko, Mykhaylo
1 / 13 shared
Kvashnina, Kristina O.
1 / 6 shared
Levytskyi, Volodymyr
1 / 8 shared
Rafaja, David
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Akselrud, Lev
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Leithe-Jasper, Andreas
1 / 6 shared
Gumeniuk, Roman
1 / 6 shared
Kainzbauer, Peter
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Terzieff, Peter
1 / 1 shared
Ipser, Herbert
1 / 23 shared
Marker, Martin C. J.
1 / 3 shared
Richter, Klaus W.
1 / 51 shared
Chart of publication period
2021
2018

Co-Authors (by relevance)

  • Eng, Lukas
  • Amber, Zeeshan H.
  • Kaiser, Martin
  • Prots, Yurii
  • Höhn, Peter
  • Jesche, Anton
  • Hunger, Jens
  • Rüsing, Michael
  • Jach, Franziska
  • Ruck, Michael
  • Wagner, Frank R.
  • Wagler, Jörg
  • Feig, Manuel
  • Motylenko, Mykhaylo
  • Kvashnina, Kristina O.
  • Levytskyi, Volodymyr
  • Rafaja, David
  • Akselrud, Lev
  • Leithe-Jasper, Andreas
  • Gumeniuk, Roman
  • Kainzbauer, Peter
  • Terzieff, Peter
  • Ipser, Herbert
  • Marker, Martin C. J.
  • Richter, Klaus W.
OrganizationsLocationPeople

article

Tricyanidoferrates(−IV) and Ruthenates(−IV) with Non-Innocent Cyanido Ligands

  • Eng, Lukas
  • Amber, Zeeshan H.
  • Kaiser, Martin
  • Prots, Yurii
  • Höhn, Peter
  • Bobnar, Matej
  • Jesche, Anton
  • Hunger, Jens
  • Rüsing, Michael
  • Jach, Franziska
  • Ruck, Michael
  • Wagner, Frank R.
Abstract

<p>Exceptionally electron-rich, nearly trigonal-planar tricyanidometalate anions [Fe(CN)<sub>3</sub>]<sup>7−</sup> and [Ru(CN)<sub>3</sub>]<sup>7−</sup> were stabilized in LiSr<sub>3</sub>[Fe(CN)<sub>3</sub>] and AE<sub>3.5</sub>[M(CN)<sub>3</sub>] (AE=Sr, Ba; M=Fe, Ru). They are the first examples of group 8 elements with the oxidation state of −IV. Microcrystalline powders were obtained by a solid-state route, single crystals from alkali metal flux. While LiSr<sub>3</sub>[Fe(CN)<sub>3</sub>] crystallizes in P6<sub>3</sub>/m, the polar space group P6<sub>3</sub> with three-fold cell volume for AE<sub>3.5</sub>[M(CN)<sub>3</sub>] is confirmed by second harmonic generation. X-ray diffraction, IR and Raman spectroscopy reveal longer C−N distances (124–128 pm) and much lower stretching frequencies (1484–1634 cm<sup>−1</sup>) than in classical cyanidometalates. Weak C−N bonds in combination with strong M−C π-bonding is a scheme also known for carbonylmetalates. Instead of the formal notation [Fe<sup>−IV</sup>(CN<sup>−</sup>)<sub>3</sub>]<sup>7−</sup>, quantum chemical calculations reveal non-innocent intermediate-valent CN<sup>1.67−</sup> ligands and a closed-shell d<sup>10</sup> configuration for Fe, that is, Fe<sup>2−</sup>.</p>

Topics
  • impedance spectroscopy
  • single crystal
  • x-ray diffraction
  • Raman spectroscopy
  • space group
  • Alkali metal