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article
Single-Crystal X-Ray Diffraction Study of Pressure and Temperature-Induced Spin Trapping in a Bistable Iron(II) Hofmann Framework
Abstract
<p>High-pressure single-crystal X-ray diffraction has been used to trap both the low-spin (LS) and high-spin (HS) states of the iron(II) Hofmann spin crossover framework, [Fe<sup>II</sup>(pdm)(H<sub>2</sub>O)[Ag(CN)<sub>2</sub>]<sub>2</sub>⋅H<sub>2</sub>O, under identical experimental conditions, allowing the structural changes arising from the spin-transition to be deconvoluted from previously reported thermal effects.</p>