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| Naji, M. |
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| Motta, Antonella |
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| Aletan, Dirar |
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| Mohamed, Tarek |
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| Ertürk, Emre |
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| Taccardi, Nicola |
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| Kononenko, Denys |
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| Petrov, R. H. | Madrid |
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| Alshaaer, Mazen | Brussels |
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| Bih, L. |
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| Casati, R. |
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| Muller, Hermance |
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| Kočí, Jan | Prague |
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| Šuljagić, Marija |
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| Kalteremidou, Kalliopi-Artemi | Brussels |
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| Azam, Siraj |
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| Ospanova, Alyiya |
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| Blanpain, Bart |
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| Ali, M. A. |
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| Popa, V. |
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| Rančić, M. |
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| Ollier, Nadège |
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| Azevedo, Nuno Monteiro |
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| Landes, Michael |
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| Rignanese, Gian-Marco |
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Zheng, Jian
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (12/12 displayed)
- 2021How Surface Species Drive Product Distribution during Ammonia Oxidation: An STM and Operando APXPS Studycitations
- 2021How Surface Species Drive Product Distribution during Ammonia Oxidation : An STM and Operando APXPS Studycitations
- 2021How Surface Species Drive Product Distribution during Ammonia Oxidationcitations
- 2019Multiple Reaction Paths for CO Oxidation on a 2D SnO x Nano-Oxide on the Pt(110) Surface: Intrinsic Reactivity and Spillovercitations
- 2018Sinter-Resistant Platinum Catalyst Supported by Metal–Organic Frameworkcitations
- 2017Bridging Zirconia Nodes within a Metal-Organic Framework via Catalytic Ni-Hydroxo Clusters to Form Heterobimetallic Nanowirescitations
- 2017Methane Oxidation to Methanol Catalyzed by Cu-Oxo Clusters Stabilized in NU-1000 Metal-Organic Frameworkcitations
- 2017Ag-Vanadates/GO Nanocomposites by Aerosol-Assisted Spray Pyrolysis: Preparation and Structural and Electrochemical Characterization of a Versatile Materialcitations
- 2016VO <sub>2</sub> /V <sub>2</sub> O <sub>5</sub> :Ag Nanostructures on a DVD as Photoelectrochemical Sensorscitations
- 2016A DFT Structural Investigation of New Bimetallic PtSn x Surface Alloys Formed on the Pt(110) Surface and Their Interaction with Carbon Monoxidecitations
- 2016Cu2O/TiO2 heterostructures on a DVD as easy&cheap photoelectrochemical sensorscitations
- 2015Comparison between the Oxygen Reduction Reaction Activity of Pd<sub>5</sub>Ce and Pt<sub>5</sub>Ce: The Importance of Crystal Structurecitations
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article
Sinter-Resistant Platinum Catalyst Supported by Metal–Organic Framework
Abstract
<p>Single atoms and few-atom clusters of platinum are uniformly installed on the zirconia nodes of a metal-organic framework (MOF) NU-1000 via targeted vapor-phase synthesis. The catalytic Pt clusters, site-isolated by organic linkers, are shown to exhibit high catalytic activity for ethylene hydrogenation while exhibiting resistance to sintering up to 200 °C. In situ IR spectroscopy reveals the presence of both single atoms and few-atom clusters that depend upon synthesis conditions. Operando X-ray absorption spectroscopy and X-ray pair distribution analyses reveal unique changes in chemical bonding environment and cluster size stability while on stream. Density functional theory calculations elucidate a favorable reaction pathway for ethylene hydrogenation with the novel catalyst. These results provide evidence that atomic layer deposition (ALD) in MOFs is a versatile approach to the rational synthesis of size-selected clusters, including noble metals, on a high surface area support.</p>