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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Korte, Lars
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (14/14 displayed)
- 2023Electron contact interlayers for low‐temperature‐processed crystalline silicon solar cellscitations
- 2023New optical dispersion models for the accurate description of the electrical permittivity in direct and indirect semiconductorscitations
- 2023Field Effect Passivation in Perovskite Solar Cells by a LiF Interlayer
- 2023Ink Design Enabling Slot‐Die Coated Perovskite Solar Cells with >22% Power Conversion Efficiency, Micro‐Modules, and 1 Year of Outdoor Performance Evaluationcitations
- 2022Monolithic perovskite/silicon tandem solar cell with >29% efficiency by enhanced hole extraction
- 2022Future of n-type PV
- 2021Interface Molecular engineering for laminated monolithic perovskite/silicon tandem solar cells with 80.4% fill factorcitations
- 2020Silicon interface passivation studied by modulated surface photovoltage spectroscopycitations
- 2018Toward Annealing-Stable Molybdenum-Oxide-Based Hole-Selective Contacts For Silicon Photovoltaicscitations
- 2017It Takes Two to Tango - Double-Layer Selective Contacts in Perovskite Solar Cells for Improved Device Performance and Reduced Hysteresiscitations
- 2017Efficient light management by textured nanoimprinted layers for perovskite solar cellscitations
- 2017It Takes Two to Tango-Double-Layer Selective Contacts in Perovskite Solar Cells for Improved Device Performance and Reduced Hysteresiscitations
- 2017ITO-free metallization for interdigitated back contact silicon heterojunction solar cells
- 2017Roadmap and roadblocks for the band gap tunability of metal halide perovskitescitations
Places of action
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article
Ink Design Enabling Slot‐Die Coated Perovskite Solar Cells with >22% Power Conversion Efficiency, Micro‐Modules, and 1 Year of Outdoor Performance Evaluation
Abstract
The next technological step in the exploration of metal‐halide perovskite solar cells is the demonstration of larger‐area device prototypes under outdoor operating conditions. The authors here demonstrate that when slot‐die coating the halide perovskite layers on large areas, ribbing effects may occur but can be prevented by adjusting the precursor ink's rheological properties. For formamidinium lead triiodide (FAPbI3) precursor inks based on 2‐methoxyethanol, the ink viscosity is adjusted by adding acetonitrile (ACN) as a co‐solvent leading to smooth FAPbI3 thin‐films with high quality and layer homogeneity. For an optimized content of 46 vol% of the ACN co‐solvent, a certified steady‐state performance of 22.3% is achieved in p‐i‐n FAPbI3‐perovskite solar cells. Scaling devices to larger areas by making laser series‐interconnected mini‐modules of 12.7 cm2, a power conversion efficiency of 17.1% is demonstrated. A full year of outdoor stability testing with continuous maximum power point tracking on encapsulated devices is performed and it is demonstrated that these devices maintain close to 100% of their initial performance during winter and spring followed by a significant performance decline during warmer summer months. This work highlights the importance of the real‐condition evaluation of larger area device prototypes to validate the technological potential of halide perovskite photovoltaics. ; Chinese Scholarship Council ; HyPerCells joint Graduate School ; German Ministry of Education and Research ; Helmholtz Energy Materials Foundry http://dx.doi.org/10.13039/501100015608 ; Federal Ministry for Education and Research ; Helmholtz Association http://dx.doi.org/10.13039/501100009318 ; Peer Reviewed