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| Naji, M. |
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| Motta, Antonella |
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| Aletan, Dirar |
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| Mohamed, Tarek |
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| Ertürk, Emre |
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| Taccardi, Nicola |
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| Kononenko, Denys |
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| Petrov, R. H. | Madrid |
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| Alshaaer, Mazen | Brussels |
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| Bih, L. |
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| Casati, R. |
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| Muller, Hermance |
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| Kočí, Jan | Prague |
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| Šuljagić, Marija |
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| Kalteremidou, Kalliopi-Artemi | Brussels |
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| Azam, Siraj |
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| Ospanova, Alyiya |
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| Blanpain, Bart |
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| Ali, M. A. |
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| Popa, V. |
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| Rančić, M. |
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| Ollier, Nadège |
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| Azevedo, Nuno Monteiro |
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| Landes, Michael |
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| Rignanese, Gian-Marco |
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Huang, Wenchao
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (8/8 displayed)
- 2017Understanding charge transport in lead iodide perovskite thin-film field-effect transistorscitations
- 2017Influence of Fullerene Acceptor on the Performance, Microstructure, and Photophysics of Low Bandgap Polymer Solar Cellscitations
- 2017Isolating and quantifying the impact of domain purity on the performance of bulk heterojunction solar cellscitations
- 2016Enhancing the Optoelectronic Performance of Perovskite Solar Cells via a Textured CH3NH3PbI3 Morphologycitations
- 2016Metal Evaporation-Induced Degradation of Fullerene Acceptors in Polymer/Fullerene Solar Cellscitations
- 2016Impact of Fullerene Mixing Behavior on the Microstructure, Photophysics, and Device Performance of Polymer/Fullerene Solar Cellscitations
- 2016Enhancing the optoelectronic performance of perovskite solar cells via a textured CH3NH3PbI3 morphologycitations
- 2014Gas-assisted preparation of lead iodide perovskite films consisting of a monolayer of single crystalline grains for high efficiency planar solar cellscitations
Places of action
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article
Influence of Fullerene Acceptor on the Performance, Microstructure, and Photophysics of Low Bandgap Polymer Solar Cells
Abstract
<p>The morphology, photophysics, and device performance of solar cells based on the low bandgap polymer poly[[2,6'-4,8-di(5-ethylhexylthienyl)benzo[1,2-b;3,3-b]dithiophene]3-fluoro-2[(2-ethylhexyl)carbonyl]thieno[3,4-b]thiophenediyl (PBDTTT-EFT) (also known as PTB7-Th) blended with different fullerene acceptors: Phenyl-C<sub>61</sub>-butyric acid methyl ester (PC<sub>61</sub>BM), phenyl-C<sub>71</sub> -butyric acid methyl ester (PC<sub>71</sub>BM), or indene-C<sub>60</sub> bisadduct (ICBA) are correlated. Compared to PC<sub>71</sub> BM-based cells - which achieve a power conversion efficiency (PCE) of 9.4% - cells using ICBA achieve a higher open-circuit voltage (V<sub>OC</sub>) of 1.0 V albeit with a lower PCE of 7.1%. To understand the origin of this lower PCE, the morphology and photophysics have been thoroughly characterized. Hard and soft X-ray scattering measurements reveal that the PBDTTT-EFT:ICBA blend has a lower crystallinity, lower domain purity, and smaller domain size compared to the PBDTTT-EFT:PC<sub>71</sub>BM blend. Incomplete photoluminescence quenching is also found in the ICBA blend with transient absorption measurements showing faster recombination dynamics at short timescales. Transient photovoltage measurements highlight further differences in recombination at longer timeframes due to the more intermixed morphology of the ICBA blend. Interestingly, a mild thermal treatment improves the performance of PBDTTT-EFT:ICBA cells which is exploited in the fabrication of a homo PBDTTT-EFT:ICBA tandem solar cell with PCE of 9.0% and V<sub>OC</sub> of 1.93 V.</p>