| People | Locations | Statistics |
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| Naji, M. |
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| Motta, Antonella |
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| Aletan, Dirar |
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| Mohamed, Tarek |
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| Ertürk, Emre |
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| Taccardi, Nicola |
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| Kononenko, Denys |
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| Petrov, R. H. | Madrid |
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| Alshaaer, Mazen | Brussels |
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| Bih, L. |
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| Casati, R. |
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| Muller, Hermance |
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| Kočí, Jan | Prague |
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| Šuljagić, Marija |
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| Kalteremidou, Kalliopi-Artemi | Brussels |
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| Azam, Siraj |
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| Ospanova, Alyiya |
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| Blanpain, Bart |
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| Ali, M. A. |
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| Popa, V. |
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| Rančić, M. |
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| Ollier, Nadège |
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| Azevedo, Nuno Monteiro |
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| Landes, Michael |
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| Rignanese, Gian-Marco |
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Smulders, Maarten M. J.
Wageningen University & Research
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (12/12 displayed)
- 2023Covalent adaptable networks using boronate linkages by incorporating TetraAzaADamantanescitations
- 2023Covalent adaptable networks using boronate linkages by incorporating TetraAzaADamantanescitations
- 2023Internal hydrogen bonding of imines to control and enhance the dynamic mechanical properties of covalent adaptable networkscitations
- 2023Metal Coordination in Polyimine Covalent Adaptable Networks for Tunable Material Properties and Enhanced Creep Resistancecitations
- 2022Raman Spectroscopy Reveals Phase Separation in Imine-Based Covalent Adaptable Networkscitations
- 2022Raman Spectroscopy Reveals Phase Separation in Imine-Based Covalent Adaptable Networkscitations
- 2022Self-healing antifouling polymer brushescitations
- 2022Diblock and random antifouling bioactive polymer brushes on gold surfaces by visible-light-induced polymerization (SI-PET-RAFT) in watercitations
- 2022Self-healing antifouling polymer brushes : Effects of degree of fluorinationcitations
- 2021Zwitterionic dendrimer – Polymer hybrid copolymers for self-assembling antifouling coatingscitations
- 2021The effect of polarity on the molecular exchange dynamics in imine-based covalent adaptable networkscitations
- 2020PLL-Poly(HPMA) Bottlebrush-Based Antifouling Coatings: Three Grafting Routescitations
Places of action
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article
Diblock and random antifouling bioactive polymer brushes on gold surfaces by visible-light-induced polymerization (SI-PET-RAFT) in water
Abstract
Surface-initiated photoinduced electron-transfer-reversible addition–fragmentation chain transfer (SI-PET-RAFT) is, for the first time, used for the creation of antifouling polymer brushes on gold surfaces based on three monomers: oligo(ethylene glycol) methyl ether methacrylate (MeOEGMA), N-(2-hydroxypropyl) methacrylamide (HPMA), and carboxybetaine methacrylamide (CBMA). These coatings are subsequently characterized by X-ray photoelectron spectroscopy (XPS) and ellipsometry. The living nature of this polymerization allows for the creation of random and diblock copolymer brushes, which are based on HPMA (superb antifouling) and CBMA (good antifouling and functionalizable via activated ester chemistry). The polymer brushes demonstrate good antifouling properties against undiluted human serum, as monitored by quartz crystal microbalance with dissipation (QCM-D) and surface plasmon resonance (SPR) spectroscopy in real time. The amount of immobilization of bioactive moieties, here an antibody immobilized using N-succinimidyl ester–1-ethyl-3-(3-dimethylaminopropyl)carbodiimide hydrochloride (NHS–EDC) coupling, in the diblock and random copolymer brushes is monitored by SPR, and is analyzed with respect to the brush structure, and is shown to be superior in the diblock copolymer brush. This approach represents a scalable, robust, mild, oxygen-tolerant, and heavy-metal-free route toward the production of antifouling and functional copolymer brushes (on gold surfaces) that open up applications in biosensing and tissue engineering.