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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Zhao, B.
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (15/15 displayed)
- 2022Unravelling thermal-mechanical effects on microstructure evolution under superplastic forming conditions in a near alpha titanium alloycitations
- 2021Self-Healing Cs<sub>3</sub>Bi<sub>2</sub>Br<sub>3</sub>I<sub>6</sub> Perovskite Wafers for X-Ray Detectioncitations
- 2020Tribological behavior of three silicon nitride ceramics in dry sliding contact against Inconel 718 over a wide range of velocitiescitations
- 2020Efficient light-emitting diodes from mixed-dimensional perovskites on a fluoride interfacecitations
- 2019Insight into the Directional Thermal Transport of Hexagonal Boron Nitride Compositescitations
- 2019Triple-Cation-Based Perovskite Photocathodes with AZO Protective Layer for Hydrogen Production Applicationscitations
- 2018Growth of Nanosized Single Crystals for Efficient Perovskite Light-Emitting Diodescitations
- 2017Kinetic Control of Perovskite Thin-Film Morphology and Application in Printable Light-Emitting Diodescitations
- 2017Ultrafast carrier cooling and thermalization in lead iodide perovskite probed with two-dimensional electronic spectroscopy
- 2017High Open-Circuit Voltages in Tin-Rich Low-Bandgap Perovskite-Based Planar Heterojunction Photovoltaicscitations
- 2017High Quality Hybrid Perovskite Semiconductor Thin Films with Remarkably Enhanced Luminescence and Defect Suppression via Quaternary Alkyl Ammonium Salt Based Treatmentcitations
- 2017Ultrafast carrier thermalization in lead iodide perovskite probed with two-dimensional electronic spectroscopycitations
- 2017High Circular Polarization of Electroluminescence Achieved via Self-Assembly of a Light-Emitting Chiral Conjugated Polymer into Multidomain Cholesteric Filmscitations
- 2015Blue-Green Color Tunable Solution Processable Organolead Chloride-Bromide Mixed Halide Perovskites for Optoelectronic Applicationscitations
- 2013Electrochemical deposition of Co(Cu)/Cu multilayered nanowirescitations
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article
High Quality Hybrid Perovskite Semiconductor Thin Films with Remarkably Enhanced Luminescence and Defect Suppression via Quaternary Alkyl Ammonium Salt Based Treatment
Abstract
<jats:title>Abstract</jats:title><jats:p>Significant enhancement in the luminescence and superior photophysical properties of CH<jats:sub>3</jats:sub>NH<jats:sub>3</jats:sub>PbBr<jats:sub>3</jats:sub> thin films prepared via simple single step spin coating process involving a novel additive mediated solvent extraction step is reported. This process results in significantly lower disorder in CH<jats:sub>3</jats:sub>NH<jats:sub>3</jats:sub>PbBr<jats:sub>3</jats:sub> perovskites with Urbach energies reducing from ≈35 to ≈17 meV, which is the lowest reported value to date. The additive mediated process also results in a remarkable improvement in the photoluminescence quantum yields (PLQYs) from 1% to 30%. Coupled with the overall increase in surface roughness, a significant increase in the internal PLQY from 7% to 77% is estimated, indicating the superior quality of the treated thin films. The resultant high quality CH<jats:sub>3</jats:sub>NH<jats:sub>3</jats:sub>PbBr<jats:sub>3</jats:sub> perovskites with remarkable photophysical properties can be used in realizing highly efficient optoelectronic devices. Highly efficient light emitting diodes using these perovskites are demonstrated here.</jats:p>