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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Unger, Eva
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (26/26 displayed)
- 2024Optical Analysis of Perovskite III-V Nanowires Interpenetrated Tandem Solar Cellscitations
- 2024Investigation of perovskite layer growth from solution on textured substrates
- 2024Bicolour, large area, inkjet-printed metal halide perovskite light emitting diodes†
- 2024Integration of Multijunction Absorbers and Catalysts for Efficient Solar‐Driven Artificial Leaf Structures: A Physical and Materials Science Perspectivecitations
- 2023Chloride-Based Additive Engineering for Efficient and Stable Wide-Bandgap Perovskite Solar Cellscitations
- 2023Large area inkjet-printed metal halide perovskite LEDs enabled by gas flow assisted drying and crystallization
- 2023Chloride‐Based Additive Engineering for Efficient and Stable Wide‐Bandgap Perovskite Solar Cellscitations
- 2023Ink Design Enabling Slot‐Die Coated Perovskite Solar Cells with >22% Power Conversion Efficiency, Micro‐Modules, and 1 Year of Outdoor Performance Evaluationcitations
- 2022An open-access database and analysis tool for perovskite solar cells based on the FAIR data principlescitations
- 2022Multi‐Stage Phase‐Segregation of Mixed Halide Perovskites under Illumination: A Quantitative Comparison of Experimental Observations and Thermodynamic Modelscitations
- 2021An open-access database and analysis tool for perovskite solar cells based on the FAIR data principlescitations
- 2021Stability assessment of p-i-n perovskite photovoltaic mini-modules utilizing different top metal electrodescitations
- 2021Roadmap on organic-inorganic hybrid perovskite semiconductors and devicescitations
- 2021Inducing ferroelastic domains in single-crystal CsPbBr3 perovskite nanowires using atomic force microscopycitations
- 2021Inducing ferroelastic domains in single-crystal CsPbBr3 perovskite nanowires using atomic force microscopycitations
- 2021Vertically Aligned CsPbBr3 Nanowire Arrays with Template-Induced Crystal Phase Transition and Stabilitycitations
- 2021Compositional and Interfacial Engineering Yield High-Performance and Stable p-i-n Perovskite Solar Cells and Mini-Modulescitations
- 2021Photoinduced energy-level realignment at interfaces between organic semiconductors and metal-halide perovskitescitations
- 2021Using Combinatorial Inkjet Printing for Synthesis and Deposition of Metal Halide Perovskites in Wavelength‐Selective Photodetectors
- 2020In Situ Imaging of Ferroelastic Domain Dynamics in CsPbBr3Perovskite Nanowires by Nanofocused Scanning X-ray Diffractioncitations
- 2020The Role of Grain Boundaries on Ionic Defect Migration in Metal Halide Perovskitescitations
- 2020Hybrid perovskite crystallization from binary solvent mixtures: interplay of evaporation rate and binding strength of solventscitations
- 2020Perovskite solar cell performance assessmentcitations
- 2020Interdependence of photon upconversion performance and antisolvent processing in thin-film halide perovskite-sensitized triplet–triplet annihilatorscitations
- 2020In situ imaging of ferroelastic domain dynamics in CsPbBr3perovskite nanowires by nanofocused scanning X-ray diffractioncitations
- 2015Enhanced Organo-Metal Halide Perovskite Photoluminescence from Nanosized Defect-Free Crystallites and Emitting Sitescitations
Places of action
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article
Chloride‐Based Additive Engineering for Efficient and Stable Wide‐Bandgap Perovskite Solar Cells
Abstract
<jats:title>Abstract</jats:title><jats:p>Metal halide perovskite based tandem solar cells are promising to achieve power conversion efficiency beyond the theoretical limit of their single‐junction counterparts. However, overcoming the significant open‐circuit voltage deficit present in wide‐bandgap perovskite solar cells remains a major hurdle for realizing efficient and stable perovskite tandem cells. Here, a holistic approach to overcoming challenges in 1.8 eV perovskite solar cells is reported by engineering the perovskite crystallization pathway by means of chloride additives. In conjunction with employing a self‐assembled monolayer as the hole‐transport layer, an open‐circuit voltage of 1.25 V and a power conversion efficiency of 17.0% are achieved. The key role of methylammonium chloride addition is elucidated in facilitating the growth of a chloride‐rich intermediate phase that directs crystallization of the desired cubic perovskite phase and induces more effective halide homogenization. The as‐formed 1.8 eV perovskite demonstrates suppressed halide segregation and improved optoelectronic properties.</jats:p>