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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Cinchetti, Mirko
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (20/20 displayed)
- 2024Carbon / Hexagons on Rectangles: Epitaxial Graphene on Rucitations
- 2023Ultrafast Coherent THz Lattice Dynamics Coupled to Spins in the van der Waals Antiferromagnet FePS3citations
- 2023Enhancing electron correlation at a 3D ferromagnetic surfacecitations
- 2023Ultrafast coherent THz lattice dynamics coupled to spins in the van der Waals antiferromagnet FePS3citations
- 2022Ultrafast coherent THz lattice dynamics coupled to spins in the van der Waals antiferromagnet FePS3
- 2022Enhancing electron correlation at a 3d ferromagnetic surfacecitations
- 2021Room-temperature on-spin-switching and tuning in a porphyrin-based multifunctional interface
- 2021Extremely low-energy ARPES of quantum well states in cubic-GaN/AlN and GaAs/AlGaAs heterostructurescitations
- 2021Room‐Temperature On‐Spin‐Switching and Tuning in a Porphyrin‐Based Multifunctional Interfacecitations
- 2020Enhancing light emission in interface engineered spin-OLEDs through spin-polarized injection at high voltagescitations
- 2020Vertical bonding distances and interfacial band structure of PTCDA on a Sn-Ag surface alloycitations
- 2018Adsorption-induced pyramidal distortion of the trimetallic nitride core inside the endohedral fullerene Sc 3 N @ C 80 on the Ag(111) surfacecitations
- 2018Induced versus intrinsic magnetic moments in ultrafast magnetization dynamicscitations
- 2017Cavity-assisted ultrafast long-range periodic energy transfer between plasmonic nanoantennascitations
- 2016Adsorption heights and bonding strength of organic molecules on a Pb-Ag surface alloycitations
- 2016Light Localization and Magneto-Optic Enhancement in Ni Antidot Arrayscitations
- 2015Topological states on the gold surfacecitations
- 2014Subpicosecond magnetization dynamics in TbCo alloyscitations
- 2013Energy-resolved magnetic domain imaging in TbCo alloys by valence band photoemission magnetic circular dichroismcitations
- 2013Spin-dependent electronic structure of the Co/Al(OP)3 interfacecitations
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article
Enhancing electron correlation at a 3d ferromagnetic surface
Abstract
Spin-resolved momentum microscopy and theoretical calculations are combined beyond the one-electron approximation to unveil the spin-dependent electronic structure of the interface formed between iron (Fe) and an ordered oxygen (O) atomic layer, and an adsorbate-induced enhancement of electronic correlations is found. It is demonstrated that this enhancement is responsible for a drastic narrowing of the Fe d-bands close to the Fermi energy (EF) and a reduction of the exchange splitting, which is not accounted for in the Stoner picture of ferromagnetism. In addition, correlation leads to a significant spin-dependent broadening of the electronic bands at higher binding energies and their merging with satellite features, which are manifestations of a pure many-electron behavior. Overall, adatom adsorption can be used to vary the material parameters of transition metal surfaces to access different intermediate electronic correlated regimes, which will otherwise not be accessible. The results show that the concepts developed to understand the physics and chemistry of adsorbate–metal interfaces, relevant for a variety of research areas, from spintronics to catalysis, need to be reconsidered with many-particle effects being of utmost importance. These may affect chemisorption energy, spin transport, magnetic order, and even play a key role in the emergence of ferromagnetism at interfaces between non-magnetic systems.