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Sheelamanthula, Rajendar
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Publications (7/7 displayed)
- 2024Flexible switch matrix addressable electrode arrays with organic electrochemical transistor and pn diode technologycitations
- 2023An ordered, self-assembled nanocomposite with efficient electronic and ionic transport.citations
- 2023Controlling swelling in mixed transport polymers through alkyl side-chain physical cross-linking.citations
- 2022Oligoethylene Glycol Side Chains Increase Charge Generation in Organic Semiconductor Nanoparticles for Enhanced Photocatalytic Hydrogen Evolutioncitations
- 2021Regiochemistry-driven organic electrochemical transistor performance enhancement in ethylene glycol-functionalized polythiophenescitations
- 2020Side Chain Redistribution as a Strategy to Boost Organic Electrochemical Transistor Performance and Stabilitycitations
- 2020Side Chain Redistribution as a Strategy to Boost Organic Electrochemical Transistor Performance and Stability.citations
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article
Side Chain Redistribution as a Strategy to Boost Organic Electrochemical Transistor Performance and Stability.
Abstract
A series of glycolated polythiophenes for use in organic electrochemical transistors (OECTs) is designed and synthesized, differing in the distribution of their ethylene glycol chains that are tethered to the conjugated backbone. While side chain redistribution does not have a significant impact on the optoelectronic properties of the polymers, this molecular engineering strategy strongly impacts the water uptake achieved in the polymers. By careful optimization of the water uptake in the polymer films, OECTs with unprecedented steady-state performances in terms of [muC* ] and current retentions up to 98% over 700 electrochemical switching cycles are developed.