| People | Locations | Statistics |
|---|---|---|
| Naji, M. |
| |
| Motta, Antonella |
| |
| Aletan, Dirar |
| |
| Mohamed, Tarek |
| |
| Ertürk, Emre |
| |
| Taccardi, Nicola |
| |
| Kononenko, Denys |
| |
| Petrov, R. H. | Madrid |
|
| Alshaaer, Mazen | Brussels |
|
| Bih, L. |
| |
| Casati, R. |
| |
| Muller, Hermance |
| |
| Kočí, Jan | Prague |
|
| Šuljagić, Marija |
| |
| Kalteremidou, Kalliopi-Artemi | Brussels |
|
| Azam, Siraj |
| |
| Ospanova, Alyiya |
| |
| Blanpain, Bart |
| |
| Ali, M. A. |
| |
| Popa, V. |
| |
| Rančić, M. |
| |
| Ollier, Nadège |
| |
| Azevedo, Nuno Monteiro |
| |
| Landes, Michael |
| |
| Rignanese, Gian-Marco |
|
Unold, Thomas
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (42/42 displayed)
- 2024Hollow Cathode Gas Flow Sputtering of Nickel Oxide Thin Films for Hole‐Transport Layer Application in Perovskite Solar Cells
- 2023Understanding the growth mechanism of BaZrS3 chalcogenide perovskite thin films from sulfurized oxide precursors
- 2023Internal electric fields control triplet formation in halide perovskite-sensitized photon upconverters
- 2023Understanding the growth mechanism of BaZrS 3 chalcogenide perovskite thin films from sulfurized oxide precursorscitations
- 2023Understanding the growth mechanism of BaZrS<sub>3</sub> chalcogenide perovskite thin films from sulfurized oxide precursorscitations
- 2023Is Cu3-xP a Semiconductor, a Metal, or a Semimetal?citations
- 2023Is Cu 3-x P a Semiconductor, a Metal, or a Semimetal?citations
- 2023Ink Design Enabling Slot‐Die Coated Perovskite Solar Cells with >22% Power Conversion Efficiency, Micro‐Modules, and 1 Year of Outdoor Performance Evaluationcitations
- 2023Hollow Cathode Gas Flow Sputtering of Nickel Oxide Thin Films for Hole‐Transport Layer Application in Perovskite Solar Cells
- 2022Monolithic perovskite/silicon tandem solar cell with >29% efficiency by enhanced hole extraction
- 2022An open-access database and analysis tool for perovskite solar cells based on the FAIR data principlescitations
- 2022Revealing the doping density in perovskite solar cells and its impact on device performancecitations
- 2022Crystallize It before It diffusescitations
- 2022Prediction and realisation of high mobility and degenerate p-type conductivity in CaCuP thin films
- 2022Prediction and realisation of high mobility and degenerate p-type conductivity in CaCuP thin films.
- 202221.6%-efficient monolithic perovskite/Cu(In,Ga)Se2 tandem solar cells with thin conformal hole transport layers for integration on rough bottom cell surfaces
- 2022Understanding performance limiting interfacial recombination in pin Perovskite solar cellscitations
- 2022Predicting Solar Cell Performance from Terahertz and Microwave Spectroscopycitations
- 2022Predicting solar cell performance from terahertz and microwave spectroscopycitations
- 2021An open-access database and analysis tool for perovskite solar cells based on the FAIR data principlescitations
- 2021Deconvoluting Energy Transport Mechanisms in Metal Halide Perovskites Using CsPbBr3 Nanowires as a Model Systemcitations
- 2021Deconvoluting Energy Transport Mechanisms in Metal Halide Perovskites Using CsPbBr3 Nanowires as a Model Systemcitations
- 2021Comment on “Resolving spatial and energetic distributions of trap states in metal halide perovskite solar cells”citations
- 2021Pathways toward 30% Efficient Single‐Junction Perovskite Solar Cells and the Role of Mobile Ionscitations
- 2021Tuning halide perovskite energy levelscitations
- 2021Tuning halide perovskite energy levelscitations
- 2021Pathways toward 30% efficient single-junction perovskite solar cells and the role of mobile ionscitations
- 2021Compositional and Interfacial Engineering Yield High-Performance and Stable p-i-n Perovskite Solar Cells and Mini-Modulescitations
- 2021Influence of the rear interface on composition and photoluminescence yield of CZTSSe absorbers: a case for an Al 2 O 3 intermediate layercitations
- 2020Photoluminescence-based characterization of halide perovskites for photovoltaicscitations
- 2020Monitoring Charge Carrier Diffusion across a Perovskite Film with Transient Absorption Spectroscopycitations
- 2020Tuning halide perovskite energy levelscitations
- 2019The Role of Bulk and Interface Recombination in High-Efficiency Low-Dimensional Perovskite Solar Cellscitations
- 2019The impact of energy alignment and interfacial recombination on the internal and external open-circuit voltage of perovskite solar cellscitations
- 2019The Role of Bulk and Interface Recombination in High‐Efficiency Low‐Dimensional Perovskite Solar Cellscitations
- 2019High open circuit voltages in pin-type perovskite solar cells through strontium additioncitations
- 2019Low Temperature Synthesis of Stable γ-CsPbI 3 Perovskite Layers for Solar Cells Obtained by High Throughput Experimentationcitations
- 2019Highly efficient monolithic perovskite/CIGSe tandem solar cells on rough bottom cell surfacescitations
- 2018High-efficiency (Li x Cu 1− x ) 2 ZnSn(S,Se) 4 kesterite solar cells with lithium alloyingcitations
- 2015Direct insight into grain boundary reconstruction in polycrystalline Cu(In,Ga)Se 2 with atomic resolutioncitations
- 2015Defect study of Cu2ZnSn(SxSe1−x)4 thin film absorbers using photoluminescence and modulated surface photovoltage spectroscopy
- 2014Electron-beam-induced current at absorber back surfaces of Cu (In,Ga) Se2 thin-film solar cellscitations
Places of action
| Organizations | Location | People |
|---|
article
The Role of Bulk and Interface Recombination in High‐Efficiency Low‐Dimensional Perovskite Solar Cells
Abstract
<jats:title>Abstract</jats:title><jats:p>2D Ruddlesden–Popper perovskite (RPP) solar cells have excellent environmental stability. However, the power conversion efficiency (PCE) of RPP cells remains inferior to 3D perovskite‐based cells. Herein, 2D (CH<jats:sub>3</jats:sub>(CH<jats:sub>2</jats:sub>)<jats:sub>3</jats:sub>NH<jats:sub>3</jats:sub>)<jats:sub>2</jats:sub>(CH<jats:sub>3</jats:sub>NH<jats:sub>3</jats:sub>)<jats:italic><jats:sub>n</jats:sub></jats:italic><jats:sub>−1</jats:sub>Pb<jats:italic><jats:sub>n</jats:sub></jats:italic>I<jats:sub>3</jats:sub><jats:italic><jats:sub>n</jats:sub></jats:italic><jats:sub>+1</jats:sub> perovskite cells with different numbers of [PbI<jats:sub>6</jats:sub>]<jats:sup>4−</jats:sup> sheets (<jats:italic>n</jats:italic> = 2–4) are analyzed. Photoluminescence quantum yield (PLQY) measurements show that nonradiative open‐circuit voltage (<jats:italic>V</jats:italic><jats:sub>OC</jats:sub>) losses outweigh radiative losses in materials with <jats:italic>n</jats:italic> > 2. The <jats:italic>n</jats:italic> = 3 and <jats:italic>n</jats:italic> = 4 films exhibit a higher PLQY than the standard 3D methylammonium lead iodide perovskite although this is accompanied by increased interfacial recombination at the top perovskite/C<jats:sub>60</jats:sub> interface. This tradeoff results in a similar PLQY in all devices, including the <jats:italic>n</jats:italic> = 2 system where the perovskite bulk dominates the recombination properties of the cell. In most cases the quasi‐Fermi level splitting matches the device <jats:italic>V</jats:italic><jats:sub>OC</jats:sub> within 20 meV, which indicates minimal recombination losses at the metal contacts. The results show that poor charge transport rather than exciton dissociation is the primary reason for the reduction in fill factor of the RPP devices. Optimized <jats:italic>n</jats:italic> = 4 RPP solar cells had PCEs of 13% with significant potential for further improvements.</jats:p>