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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Vaynzof, Yana
Leibniz Institute for Solid State and Materials Research
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (31/31 displayed)
- 2024Photoluminescence Mapping over Laser Pulse Fluence and Repetition Rate as a Fingerprint of Charge and Defect Dynamics in Perovskitescitations
- 2024SnS2 Thin Film with In Situ and Controllable Sb Doping via Atomic Layer Deposition for Optoelectronic Applicationscitations
- 2024Tuning Phase Purity in Chiral 2D Perovskitescitations
- 2024Ultrafast vibrational control of organohalide perovskite optoelectronic devices using vibrationally promoted electronic resonancecitations
- 2024Distributed Feedback Lasing in Thermally Imprinted Phase‐Stabilized CsPbI3 Thin Filmscitations
- 2024Charge Trapping and Defect Dynamics as Origin of Memory Effects in Metal Halide Perovskite Memlumorscitations
- 2024Eco‐Friendly Approach to Ultra‐Thin Metal Oxides‐ Solution Sheared Aluminum Oxide for Half‐Volt Operation of Organic Field‐Effect Transistorscitations
- 2024Eco‐Friendly Approach to Ultra‐Thin Metal Oxides‐ Solution Sheared Aluminum Oxide for Half‐Volt Operation of Organic Field‐Effect Transistorscitations
- 2024From Chalcogen Bonding to S–π Interactions in Hybrid Perovskite Photovoltaicscitations
- 2023Band Structure Engineering in Highly Crystalline Organic Semiconductorscitations
- 2023Photoluminescence Mapping over Laser Pulse Fluence and Repetition Rate as a Fingerprint of Charge and Defect Dynamics in Perovskites
- 2023Solvent-antisolvent interactions in metal halide perovskites
- 2023Elucidating Structure Formation in Highly Oriented Triple Cation Perovskite Filmscitations
- 2023Remarkable performance recovery in highly defective perovskite solar cells by photo-oxidationcitations
- 2023Confinement and exciton binding energy effects on hot carrier cooling in lead halide perovskite nanomaterialscitations
- 2023Confinement and exciton binding energy effects on hot carrier cooling in lead halide perovskite nanomaterialscitations
- 2023Influence of chemical interactions on the electronic properties of BiOI/organic semiconductor heterojunctions for application in solution-processed electronics
- 2022Structural colors with embedded anti-counterfeit features fabricated by laser-based methodscitations
- 2022High‐Efficiency Perovskite–Organic Blend Light‐Emitting Diodes Featuring Self‐Assembled Monolayers as Hole‐Injecting Interlayerscitations
- 2022Effects of sub-picosecond direct laser interference patterning on the optoelectronic properties of fluorine-doped tin oxide thin filmscitations
- 2021Roadmap on organic-inorganic hybrid perovskite semiconductors and devicescitations
- 2021Ruddlesden-Popper-Phase Hybrid Halide Perovskite/Small-Molecule Organic Blend Memory Transistorscitations
- 2021Are Shockley-Read-Hall and ABC models valid for lead halide perovskites?citations
- 2021Electrical Pumping of Perovskite Diodes: Toward Stimulated Emission.
- 2020Inkjet‐Printed Micrometer‐Thick Perovskite Solar Cells with Large Columnar Grains
- 2019Inkjet‐Printed Micrometer‐Thick Perovskite Solar Cells with Large Columnar Grainscitations
- 2019The effect of side-chain length on the microstructure and processing window of zone-cast naphthalene-based bispentalenescitations
- 2018Electroluminescence from Solution-Processed Pinhole-Free Nanometer-Thickness Layers of Conjugated Polymers.
- 2016Efficient perovskite solar cells by metal ion dopingcitations
- 2015Role of PbSe Structural Stabilization in Photovoltaic Cellscitations
- 2014Performance and Stability Enhancement of Dye-Sensitized and Perovskite Solar Cells by Al Doping of TiO2citations
Places of action
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article
Distributed Feedback Lasing in Thermally Imprinted Phase‐Stabilized CsPbI3 Thin Films
Abstract
<jats:title>Abstract</jats:title><jats:p>All‐inorganic cesium lead halide perovskites (CsPbX<jats:sub>3</jats:sub>, with X = I, Br, Cl) are of great interest for light‐emitting diodes and lasers, as they promise improved thermal stability compared to their organic–inorganic analogues. However, among this family of materials, CsPbI<jats:sub>3</jats:sub> shows a detrimental phase instability that causes the perovskite to convert to a thermodynamically preferred non‐perovskite phase (yellow phase) at room temperature. In fact, reports on lasers using thin films of CsPbI<jats:sub>3</jats:sub> as gain medium are missing, as of yet. Here, the first distributed feedback (DFB) lasers based on CsPbI<jats:sub>3</jats:sub> thin films are presented with a resonator directly patterned into the perovskite by thermal nanoimprint. This breakthrough is unlocked by the additive polyvinyl pyrrolidone (PVP), that affords the formation of perovskite layers consisting of phase stable γ‐CsPbI<jats:sub>3</jats:sub> nanocrystals, that are even preserved during thermal imprint at 170 °C. The DFB lasers show a low lasing threshold of 45 µJ cm<jats:sup>−2</jats:sup> at room temperature under optical pumping and a tunable emission in the deep red spectral region between 714.1 to 723.4 nm. It is anticipated that the findings of this work will have a broad relevance for future electrically driven perovskite lasers and for light‐emitting diodes based on CsPbI<jats:sub>3</jats:sub> as active medium.</jats:p>