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| Naji, M. |
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| Motta, Antonella |
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| Aletan, Dirar |
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| Mohamed, Tarek |
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| Ertürk, Emre |
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| Taccardi, Nicola |
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| Kononenko, Denys |
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| Petrov, R. H. | Madrid |
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| Alshaaer, Mazen | Brussels |
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| Bih, L. |
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| Casati, R. |
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| Muller, Hermance |
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| Kočí, Jan | Prague |
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| Šuljagić, Marija |
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| Kalteremidou, Kalliopi-Artemi | Brussels |
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| Azam, Siraj |
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| Ospanova, Alyiya |
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| Blanpain, Bart |
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| Ali, M. A. |
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| Popa, V. |
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| Rančić, M. |
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| Ollier, Nadège |
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| Azevedo, Nuno Monteiro |
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| Landes, Michael |
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| Rignanese, Gian-Marco |
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Yan, Feng
University of Manchester
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (9/9 displayed)
- 2024Understanding the Surface Chemistry of SnO 2 Nanoparticles for High Performance and Stable Organic Solar Cellscitations
- 2024Use of carbon electrodes to reduce mobile ion concentration and improve reliability of metal halide perovskite photovoltaicscitations
- 2024Understanding the Surface Chemistry of SnO2 Nanoparticles for High Performance and Stable Organic Solar Cellscitations
- 2023Temperature-responsive and biocompatible nanocarriers based on clay nanotubes for controlled anti-cancer drug releasecitations
- 2023Effect of intermolecular interactions on the glass transition temperature of chemically modified alternating polyketonescitations
- 2023Effect of intermolecular interactions on the glass transition temperature of chemically modified alternating polyketonescitations
- 2022Optimizing inference serving on serverless platformscitations
- 2018p‐Doping of Copper(I) Thiocyanate (CuSCN) Hole‐Transport Layers for High‐Performance Transistors and Organic Solar Cellscitations
- 2014Physicochemical properties of 1,2,4-triazolium perfluorobutanesulfonate as an archetypal pure protic organic ionic plastic crystal electrolyte
Places of action
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article
Understanding the Surface Chemistry of SnO2 Nanoparticles for High Performance and Stable Organic Solar Cells
Abstract
<p>In organic solar cells, the interfaces between the photoactive layer and the transport layers are critical in determining not only the efficiency but also their stability. When solution-processed metal oxides are employed as the electron transport layer, the presence of surface defects can downgrade the charge extraction, lowering the photovoltaic parameters. Thus, understanding the origin of these defects is essential to prevent their detrimental effects. Herein, it is shown that a widely reported and commercially available colloidal SnO<sub>2</sub> dispersion leads to suboptimal interfaces with the organic layer, as evidenced by the s-shaped J–V curves and poor stability. By investigating the SnO<sub>2</sub> surface chemistry, the presence of potassium ions as stabilizing ligands is identified. By removing them with a simple washing with deionized water, the s-shape is removed and the short-circuit current is improved. It is tested for two prototypical blends, TPD-3F:IT-4F and PM6:L8:BO, and for both the power conversion efficiency is improved up to 12.82% and 16.26%, from 11.06% and 15.17% obtained with the pristine SnO<sub>2</sub>, respectively. More strikingly, the stability is strongly correlated with the surface ions concentration, and these improved devices maintain ≈87% and ≈85% of their initial efficiency after 100 h of illumination for TPD-3F:IT-4F and PM6:L8:BO, respectively.</p>