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| Naji, M. |
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| Motta, Antonella |
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| Aletan, Dirar |
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| Mohamed, Tarek |
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| Ertürk, Emre |
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| Taccardi, Nicola |
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| Kononenko, Denys |
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| Petrov, R. H. | Madrid |
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| Alshaaer, Mazen | Brussels |
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| Bih, L. |
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| Casati, R. |
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| Muller, Hermance |
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| Kočí, Jan | Prague |
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| Šuljagić, Marija |
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| Kalteremidou, Kalliopi-Artemi | Brussels |
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| Azam, Siraj |
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| Ospanova, Alyiya |
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| Blanpain, Bart |
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| Ali, M. A. |
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| Popa, V. |
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| Rančić, M. |
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| Ollier, Nadège |
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| Azevedo, Nuno Monteiro |
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| Landes, Michael |
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| Rignanese, Gian-Marco |
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Mayer, Joachim
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (30/30 displayed)
- 2024The effect of Laves phases and nano-precipitates on the electrochemical corrosion resistance of Mg-Al-Ca alloys under alkaline conditionscitations
- 2024Natural and artificial aging behaviour of Al-Cu-Mg-Ag-Ti-B (A205) alloy processed by laser powder bed fusion: Strengthening mechanisms and failure analysiscitations
- 2023Improved Route to Linear Triblock Copolymers by Coupling with Glycidyl Ether-Activated Poly(ethylene oxide) Chainscitations
- 2023Three-dimensional printing of silica glass with sub-micrometer resolutioncitations
- 2023Three-dimensional printing of silica glass with sub-micrometer resolutioncitations
- 2023Microstructure stability and self-diffusion in the equiatomic HfScTiZr HCP multi-principal element alloycitations
- 2023Role of Fe/Co Ratio in Dual Phase Ce0.8Gd0.2O2−δ–Fe3−xCoxO4 Composites for Oxygen Separationcitations
- 2023Mechanistic study of dark etching regions in bearing steels due to rolling contact fatiguecitations
- 2023Mechanistic study of dark etching regions in bearing steels due to rolling contact fatiguecitations
- 2023Laves phases in Mg-Al-Ca alloys and their effect on mechanical properties
- 2023Coherent twin-oriented Al3Sc-based precipitates in Al matrixcitations
- 2023Development of a Bioreactor-Coupled Flow-Cell Setup for 3D In Situ Nanotomography of Mg Alloy Biodegradationcitations
- 2022Residual Stress Reduction with the LTT Effect in Low Carbon Manganese-Steel through Chemical Composition Manipulation Using Dissimilar Filler Material in Laser Beam Weldingcitations
- 2022Simulation of the fatigue crack initiation in SAE 52100 martensitic hardened bearing steel during rolling contact
- 2022Elucidation of formation and transformation mechanisms of Ca-rich Laves phase in Mg-Al-Ca-Mn alloyscitations
- 2022Proximity-induced superconductivity in (Bi1−xSbx)2Te3 topological-insulator nanowirescitations
- 2021Measurement of polarization effects in dual-phase ceria-based oxygen permeation membranes using Kelvin probe force microscopycitations
- 2021Investigation of Alloy‐Dependent Occurrence of Ferromagnetism in Carbon‐Expanded Austenitic Steel after Low‐Temperature Surface Hardening
- 2021Temperature dependent partitioning mechanisms and its associated microstructural evolution in a CMnSiAl quenching and partitioning (Q&P) steelcitations
- 2021Atomic Structure and Electron Magnetic Circular Dichroism of Individual Rock Salt Structure Antiphase Boundaries in Spinel Ferritescitations
- 2021Structural Phase Transition and In-Situ Energy Storage Pathway in Nonpolar Materials: A Reviewcitations
- 2020Antiphase Boundaries Constitute Fast Cation Diffusion Paths in SrTiO3 Memristive Devices
- 2020Antiphase Boundaries Constitute Fast Cation Diffusion Paths in SrTiO3 Memristive Devicescitations
- 2020Combined κ-carbide precipitation and recovery enables ultra-high strength and ductility in light-weight steelscitations
- 2020A Nanoscale Study of Thermally Grown Chromia on High-Cr Ferritic Steels and Associated Oxidation Mechanismscitations
- 2017Electron microscopy investigations of microstructural alterations due to classical Rolling Contact Fatigue (RCF) in martensitic AISI 52100 bearing steelcitations
- 2017Microstructural changes in White Etching Cracks (WECs) and their relationship with those in Dark Etching Region (DER) and White Etching Bands (WEBs) due to Rolling Contact Fatigue (RCF)citations
- 2016MOVPE and characterization of rhombohedral Ge1Sb2Te4/Si(111)
- 2011Au@Hg Nanoalloy Formation Through Direct Amalgamation: Structural, Spectroscopic, and Computational Evidence for Slow Nanoscale Diffusioncitations
- 2008Novel carbon nanosheets as support for ultrahigh-resolution structural analysis of nanoparticlescitations
Places of action
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document
Antiphase Boundaries Constitute Fast Cation Diffusion Paths in SrTiO3 Memristive Devices
Abstract
<p>Resistive switching in transition metal oxide-based metal-insulator-metal structures relies on the reversible drift of ions under an applied electric field on the nanoscale. In such structures, the formation of conductive filaments is believed to be induced by the electric-field driven migration of oxygen anions, while the cation sublattice is often considered to be inactive. This simple mechanistic picture of the switching process is incomplete as both oxygen anions and metal cations have been previously identified as mobile species under device operation. Here, spectromicroscopic techniques combined with atomistic simulations to elucidate the diffusion and drift processes that take place in the resistive switching model material SrTiO<sub>3</sub> are used. It is demonstrated that the conductive filament in epitaxial SrTiO<sub>3</sub> devices is not homogenous but exhibits a complex microstructure. Specifically, the filament consists of a conductive Ti<sup>3+</sup>-rich region and insulating Sr-rich islands. Transmission electron microscopy shows that the Sr-rich islands emerge above Ruddlesden–Popper type antiphase boundaries. The role of these extended defects is clarified by molecular static and molecular dynamic simulations, which reveal that the Ruddlesden–Popper antiphase boundaries constitute diffusion fast-paths for Sr cations in the perovskites structure.</p>