| People | Locations | Statistics |
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| Naji, M. |
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| Motta, Antonella |
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| Aletan, Dirar |
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| Mohamed, Tarek |
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| Ertürk, Emre |
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| Taccardi, Nicola |
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| Kononenko, Denys |
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| Petrov, R. H. | Madrid |
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| Alshaaer, Mazen | Brussels |
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| Bih, L. |
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| Casati, R. |
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| Muller, Hermance |
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| Kočí, Jan | Prague |
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| Šuljagić, Marija |
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| Kalteremidou, Kalliopi-Artemi | Brussels |
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| Azam, Siraj |
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| Ospanova, Alyiya |
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| Blanpain, Bart |
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| Ali, M. A. |
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| Popa, V. |
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| Rančić, M. |
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| Ollier, Nadège |
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| Azevedo, Nuno Monteiro |
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| Landes, Michael |
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| Rignanese, Gian-Marco |
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Mann, Stephen
University of Bristol
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (25/25 displayed)
- 2020Mixed liposomes containing gram-positive bacteria lipidscitations
- 2017Self-Assembly of Colloidal Nanocomposite Hydrogels Using 1D Cellulose Nanocrystals and 2D Exfoliated Organoclay Layerscitations
- 2015Multimodal Plasmonics in Fused Colloidal Networkscitations
- 2014In situ X-ray reflectivity studies of molecular and molecular-cluster intercalation within purple membrane filmscitations
- 2014In situ X-ray reflectivity studies of molecular and molecular-cluster intercalation within purple membrane filmscitations
- 2014Molecular dynamics simulations reveal a dielectric-responsive coronal structure in protein-polymer surfactant hybrid nanoconstructscitations
- 2013Electrochemical crystallization of spatially organized copper microwire arrays within biomineralized (dentine) templatescitations
- 2013Apoferritin-encapsulated PbS quantum dots significantly inhibit growth of colorectal carcinoma cellscitations
- 2013Apoferritin-encapsulated PbS quantum dots significantly inhibit growth of colorectal carcinoma cellscitations
- 2013Directing Chondrogenesis of Stem Cells with Specific Blends of Cellulose and Silkcitations
- 2013The reinforcement effects of graphene oxide nanoplatelets on the mechanical and viscoelastic properties of natural rubber
- 2012High magnetic field quantum transport in Au nanoparticle-cellulose filmscitations
- 2012Polymer/nucleotide droplets as bio-inspired functional micro-compartmentscitations
- 2012The differential effect of apoferritin-PbS nanocomposites on cell cycle progression in normal and cancerous cellscitations
- 2011Lamellar nanocomposite films of purple membrane and poly(acrylate)
- 2011Guest-Molecule-Directed Assembly of Mesostructured Nanocomposite Polymer/Organoclay Hydrogelscitations
- 2011Supramolecular hydrogels derived from silver ion-mediated self-assembly of 5 '-guanosine monophosphatecitations
- 2010Assembly of poly(methacrylate)/purple membrane lamellar nanocomposite films by intercalation and in situ polymerisationcitations
- 2009Structure and Properties of Silicified Purple Membrane Thin Filmscitations
- 2009Hydroxyapatite pattern formation in PVA gelscitations
- 2009Membrane stabilization and transformation in organoclay-vesicle hybrid constructscitations
- 2009Immobilisation and encapsulation of functional protein-inorganic constructscitations
- 2007Bio-functional mesolamellar nanocomposites based on inorganic/polymer intercalation in purple membrane (bacteriorhodopsin) filmscitations
- 2007Biomimetic hydroxyapatite-drug nanocrystals as potential bone substitutes with antitumor drug delivery propertiescitations
- 2007Influence of polymer co-intercalation on guest release from aminopropyl-functionalized magnesium phyllosilicate mesolamellar nanocompositescitations
Places of action
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article
Guest-Molecule-Directed Assembly of Mesostructured Nanocomposite Polymer/Organoclay Hydrogels
Abstract
Given the urgent need for soft materials with high functional value, hydrogels based on the integrative assembly of organic polymers and nanoscale inorganic building blocks-so-called nanocomposite polymer hydrogels-offer a generic approach to swollen hybrid networks with tuneable and synergistic properties. Here, we report a new approach to assembling nanocomposite polymer hydrogels with multiple levels of structural complexity and enhanced functionality by using nanoscale integration of mesostructured inorganic building blocks capable of sequestering and releasing drugs (ibuprofen, aspirin, naproxen) and enzymes (glucose oxidase). The viscoelastic materials are produced by noncovalent crosslinking of poly(vinylpyrrolidone) in the presence of low amounts (1-5 wt%) of an exfoliated synthetic organoclay that undergoes in situ guest-molecule-directed self-assembly. The hydrogels can be moulded into shape-persistent, free-standing objects that are stable between pH values of 4 to 11 and self-heal when damaged. Significantly, the mesostructured nanocomposite polymer hydrogels, which can be reversibly dried and reconstituted in the form of highly swollen materials, exhibit sustained drug release and can be recharged and reused. The results provide important guidelines for developing new multifunctional nanocomposite polymer hydrogels based on the concerted self-assembly of inorganic building blocks with mesostructured interiors.