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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Calzada, M. L.
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (24/24 displayed)
- 2023Low-temperature sol–gel methods for the integration of crystalline metal oxide thin films in flexible electronics
- 2023Evolution of the crystalline structure in (Bi0.5Na0.5)1-xBa x TiO3 thin films around the Morphotropic Phase Boundary
- 2023Low-temperature solution processing route for potassium sodium niobate (KNN) thin filmscitations
- 2022A Sustainable Self-Induced Solution Seeding Approach for Multipurpose BiFeO3 Active Layers in Flexible Electronic Devices
- 2020Photoferroelectric thin films for flexible systems by a three-in-one solution-based approach
- 2020Nanostructure stabilization by low-temperature dopant pinning in multiferroic BiFeO3-based thin films produced by aqueous chemical solution deposition
- 2019Preparation and Characterization of Large Area Li-NASICON Electrolyte Thick Filmscitations
- 2016Influence of excesses of volatile elements on structure and composition of solution derived lead-free (Bi0.50Na0.50)1xBaxTiO3 thin filmscitations
- 2016Influence of excesses of volatile elements on structure and composition of solution derived lead-free (Bi0.50Na0.50)1xBaxTiO3 thin filmscitations
- 2016Photochemical solution processing of films of metastable phases for flexible devices the β-Bi 2 O 3 polymorphcitations
- 2016Photochemical solution processing of films of metastable phases for flexible devices: the beta-Bi2O3 polymorph
- 2015Polarization switching at room temperature of undoped BiFeO3 thin films crystallized at temperatures between 400 ≤ T ≤ 500 °Ccitations
- 2014A UV-absorber bismuth(III)-N-methyldiethanolamine complex as a low-temperature precursor for bismuth-based oxide thin films
- 2011Influence of the substrate surface on the self-assembly of ferroelectric PbTiO nanostructures obtained by microemulsion assisted Chemical Solution Depositioncitations
- 2010Properties of morphotropic phase boundary Pb(Mg1/3Nb2/3)O3-PbTiO3 films with submicron range thickness on Si based substrates
- 2010Properties of morphotropic phase boundary Pb(Mg1/3Nb2/3)O3PbTiO3 films with submicrometre range thickness on Si-based substratescitations
- 2006Entirely aqueous solution-gel route for the preparation of (Pb1-xCax)TiO3 thin filmscitations
- 2005Interfacial phases and electrical characteristics of ferreoelectric strontium bismuth tantalate films on Pt/TiO2 and tTi/Pt/Ti heterostructure electrodescitations
- 2005(Pb,Ca)TiO3/(Pb,La)TiO3/(Pb,Ca)TiO3 heterostructure characterized as ferroelectric multifunctional materialcitations
- 2005Dielectric properties of Pb0.5Ca0.5TiO3 thin filmscitations
- 2004Compositional and structural study of ferroelectric multilayer (Pb,La)TiO3/(Pb,Ca)TiO3 sol-gel thin filmscitations
- 2004Raman scattering in sol-gel derived PbTiO3 films modified with Cacitations
- 2004Nanoscale properties of ferroelectric ultrathin SBT filmscitations
- 2003Microstructure and local piezoelectric properties of (Pb,Ca)TiO3 thin filmscitations
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article
Low-temperature sol–gel methods for the integration of crystalline metal oxide thin films in flexible electronics
Abstract
The development of low-temperature sol–gel (solution) processes for the fabrication of crystalline metal oxide thin films has become a key objective in the emerging Flexible Electronics. To achieve this target, crystalline oxide films need to be deposited on flexible substrates, which have degradation temperatures below 350 °C (e.g., polymers or textile). This achievement would be a step towards improving the performance of the flexible device, making feasible applications now restrained (e.g. smart-skin, flexible-displays or solar-cells) and whose performance is associated to the functional properties of the crystalline oxide (e.g., ferroelectricity, pyroelectricity or piezoelectricity). However, this is a challenge because the crystallization of these oxides usually occurs at high temperatures, over 600 °C. This paper shows an overview to the solution strategies devised in our group for the low-temperature fabrication of crystalline metal oxide thin films, mostly ferroelectric perovskites (e.g., BiFeO3, PbTiO3 or Pb(Zr,Ti)O3). We have made use of UV-light as an alternative energy source to the thermal energy conventionally used to obtain the crystalline oxide. High photosensitive sol–gel solutions have been synthesized and the solution-deposited layers irradiated with UV-excimer lamps. A precise control of the photoreactions occurring during the irradiation of these layers has been carried out with the aim of advancing the formation of a high-densified, defect-free amorphous metal oxide film that easily can be converted into crystalline at temperatures compatible with the use of polymer substrates.