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Naji, M. |
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Motta, Antonella |
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Aletan, Dirar |
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Mohamed, Tarek |
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Ertürk, Emre |
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Taccardi, Nicola |
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Kononenko, Denys |
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Petrov, R. H. | Madrid |
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Alshaaer, Mazen | Brussels |
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Bih, L. |
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Casati, R. |
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Muller, Hermance |
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Kočí, Jan | Prague |
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Šuljagić, Marija |
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Kalteremidou, Kalliopi-Artemi | Brussels |
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Azam, Siraj |
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Ospanova, Alyiya |
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Blanpain, Bart |
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Ali, M. A. |
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Popa, V. |
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Rančić, M. |
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Ollier, Nadège |
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Azevedo, Nuno Monteiro |
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Landes, Michael |
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Rignanese, Gian-Marco |
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Kumar, Jitendra
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (9/9 displayed)
- 2024Charge Trapping and Defect Dynamics as Origin of Memory Effects in Metal Halide Perovskite Memlumorscitations
- 2023An investigation of combined effect of infill pattern, density, and layer thickness on mechanical properties of 3D printed ABS by fused filament fabricationcitations
- 2022Loop Quantum Gravity motivated multihorizon rotating black holescitations
- 2022Visualization of 3D to quasi 2D conversion of perovskite thin films <i>via in situ</i> photoluminescence measurement: a facile route to design a graded energy landscapecitations
- 2020Unraveling the antisolvent dripping delay effect on the Stranski-Krastanov growth of CH3NH3PbBr3 thin films: a facile route for preparing a textured morphology with improved optoelectronic properties.
- 2020Unraveling the antisolvent dripping delay effect on the Stranski-Krastanov growth of CH<sub>3</sub>NH<sub>3</sub>PbBr<sub>3</sub> thin films: a facile route for preparing a textured morphology with improved optoelectronic propertiescitations
- 2018Mechanical hysteresis, interface and filler–filler structural breakdowns in ethylene vinyl acetate organoclay composites internally lubricated via radiolytically degraded PTFE microparticlescitations
- 2017Coordination complexes of copper(II) with herbicide-trichlorophenoxyacetate: Syntheses, characterization, single crystal X-ray structure and packing analyses of monomeric [Cu(γ-pic)3(2,4,5-trichlorophenoxyacetate)]·H2O, [trans-Cu(en)2(2,4,5-trichlorophenoxyacetate)2]·2H2O and dimeric [Cu2(H2tea)2(2,4,5-trichlorophenoxyacetate)2]·2(H2O)citations
- 2012Effect of Sheet Resistance and Morphology of ITO Thin Films on Polymer Solar Cell Characteristicscitations
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article
Unraveling the antisolvent dripping delay effect on the Stranski-Krastanov growth of CH<sub>3</sub>NH<sub>3</sub>PbBr<sub>3</sub> thin films: a facile route for preparing a textured morphology with improved optoelectronic properties
Abstract
Inorganic-organic hybrid perovskite materials have been a topic of interest for the last few years due to their superior optoelectronic properties. However, the optical properties of perovskite materials are strongly dependent on the film morphology. A textured film morphology is expected to have higher light absorption as well as light out-coupling efficiency compared to a smooth film. There have been numerous methods for controlling and optimizing the film morphology to achieve high efficiency in solar cells and light emitting diodes. Here we have demonstrated that controlled anti-solvent treatment at low temperature can lead to Stranski-Krastanov growth in CH3NH3PbBr3 thin films with superior optical and electronic properties for light emitting diode applications. We have studied their photoluminescence properties at the micro- to nano-scale via fluorescence microscopy, hyper-spectral imaging and scanning near-field optical microscopy. We have demonstrated that the nanostructured micro-islands are highly emissive because of large quasi-Fermi level splitting (QFLS) due to the localization of free charges in the smaller crystals. We have shown that the photoluminescence as well as electroluminescence can be improved by at least seven-fold due to the presence of micro-islands on a smooth background film enhancing light out-coupling. Photo-induced photoluminescence enhancement is also observed in smooth films while micro-islands show photo-degradation.