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| Naji, M. |
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| Motta, Antonella |
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| Aletan, Dirar |
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| Mohamed, Tarek |
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| Ertürk, Emre |
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| Taccardi, Nicola |
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| Kononenko, Denys |
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| Petrov, R. H. | Madrid |
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| Alshaaer, Mazen | Brussels |
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| Bih, L. |
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| Casati, R. |
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| Muller, Hermance |
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| Kočí, Jan | Prague |
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| Šuljagić, Marija |
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| Kalteremidou, Kalliopi-Artemi | Brussels |
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| Azam, Siraj |
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| Ospanova, Alyiya |
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| Blanpain, Bart |
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| Ali, M. A. |
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| Popa, V. |
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| Rančić, M. |
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| Ollier, Nadège |
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| Azevedo, Nuno Monteiro |
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| Landes, Michael |
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| Rignanese, Gian-Marco |
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Tkachenko, Nikolai V.
Tampere University
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (19/19 displayed)
- 2024Laterally Bound Co Porphyrin on CdTe QD : A Long-Lived Charge-Separated Nanocompositecitations
- 2024Contactless analysis of surface passivation and charge transfer at the TiO 2-Si interfacecitations
- 2024Contactless analysis of surface passivation and charge transfer at the TiO 2-Si interfacecitations
- 2024Transient Absorption Spectroscopy of Filmscitations
- 2024Contactless analysis of surface passivation and charge transfer at the TiO2-Si interfacecitations
- 2023Laterally Bound Co Porphyrin on CdTe QD : A Long-Lived Charge-Separated Nanocompositecitations
- 2023Is Carrier Mobility a Limiting Factor for Charge Transfer in Tio2/Si Devices? A Study by Transient Reflectance Spectroscopycitations
- 2022Tunable Ti3+-Mediated Charge Carrier Dynamics of Atomic Layer Deposition-Grown Amorphous TiO2citations
- 2021Comparison of the heat-treatment effect on carrier dynamics in TiO2 thin films deposited by different methodscitations
- 2020Optimization of photogenerated charge carrier lifetimes in ald grown tio2 for photonic applicationscitations
- 2020Monitoring Charge Carrier Diffusion across a Perovskite Film with Transient Absorption Spectroscopycitations
- 2019Multiphoton Excitation of CsPbBr3 Perovskite Quantum Dots (PQDs) : How Many Electrons Can One PQD Donate to Multiple Molecular Acceptors?citations
- 2019Electronically Coupled Uranium and Iron Oxide Heterojunctions as Efficient Water Oxidation Catalystscitations
- 2019Electronically Coupled Uranium and Iron Oxide Heterojunctions as Efficient Water Oxidation Catalystscitations
- 2019Refractive index change dominates the transient absorption response of metal halide perovskite thin films in the near infraredcitations
- 2018Critical role and modification of surface states in hematite films for enhancing oxygen evolution activitycitations
- 2017Tailored Fabrication of Transferable and Hollow Weblike Titanium Dioxide Structurescitations
- 2015Subpicosecond to Second Time-Scale Charge Carrier Kinetics in Hematite-Titania Nanocomposite Photoanodescitations
- 2015Subpicosecond to Second Time-Scale Charge Carrier Kinetics in Hematite-Titania Nanocomposite Photoanodescitations
Places of action
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article
Subpicosecond to Second Time-Scale Charge Carrier Kinetics in Hematite-Titania Nanocomposite Photoanodes
Abstract
<p>Water splitting with hematite is negatively affected by poor intrinsic charge transport properties. However, they can be modified by forming heterojunctions to improve charge separation. For this purpose, charge dynamics of TiO2:alpha-Fe2O3 nanocomposite photoanodes are studied using transient absorption spectroscopy to monitor the evolution of photogenerated charge carriers as a function of applied bias voltage. The bias affects the charge carrier dynamics, leading to trapped electrons in the submillisecond time scale and an accumulation of holes with a lifetime of 0.4 +/- 0.1 s. By contrast, slower electron trapping and only few long-lived holes are observed in a bare hematite photoanode. The decay of the long-lived holes is 1 order of magnitude faster for the composite photoanodes than previously published for doped hematite, indicative of higher catalytic efficiency. These results illustrate the advantages of using composite materials to overcome poor charge carrier dynamics, leading to a 30-fold enhancement in photocurrent.</p>