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| Naji, M. |
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| Motta, Antonella |
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| Aletan, Dirar |
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| Mohamed, Tarek |
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| Ertürk, Emre |
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| Taccardi, Nicola |
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| Kononenko, Denys |
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| Petrov, R. H. | Madrid |
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| Alshaaer, Mazen | Brussels |
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| Bih, L. |
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| Casati, R. |
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| Muller, Hermance |
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| Kočí, Jan | Prague |
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| Šuljagić, Marija |
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| Kalteremidou, Kalliopi-Artemi | Brussels |
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| Azam, Siraj |
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| Ospanova, Alyiya |
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| Blanpain, Bart |
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| Ali, M. A. |
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| Popa, V. |
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| Rančić, M. |
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| Ollier, Nadège |
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| Azevedo, Nuno Monteiro |
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| Landes, Michael |
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| Rignanese, Gian-Marco |
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Das, Amit
in Cooperation with on an Cooperation-Score of 37%
Topics
Publications (18/18 displayed)
- 2024Unlocking the Potential of Lignin: Towards a Sustainable Solution for Tire Rubber Compound Reinforcementcitations
- 2022Electrically conductive and piezoresistive polymer nanocomposites using multiwalled carbon nanotubes in a flexible copolyester: Spectroscopic, morphological, mechanical and electrical properties
- 2022Ferric Ions Crosslinked Epoxidized Natural Rubber Filled with Carbon Nanotubes and Conductive Carbon Black Hybrid Fillers
- 2021Treasuring waste lignin as superior reinforcing filler in high cis-polybutadiene rubbercitations
- 2020Friction, abrasion and crack growth behavior of in-situ and ex-situ silica filled rubber compositescitations
- 2020Verfahren zur Herstellung von Lignin-PAN-basierten Polymercompounds und Lignin-PAN-basierte Polymercompounds
- 2019Influence of Zn concentration on interfacial intermetallics during liquid and solid state reaction of hypo and hypereutectic Sn-Zn solder alloyscitations
- 2019The Taste of Waste: The Edge of Eggshell Over Calcium Carbonate in Acrylonitrile Butadiene Rubber
- 2019Devulcanization of Waste Rubber and Generation of Active Sites for Silica Reinforcement
- 2018Improved electromechanical response in acrylic rubber by different carbon-based fillerscitations
- 2018Temperature scanning stress relaxation of an autonomous self-healing elastomer containing non-covalent reversible network junctionscitations
- 2018Further enhancement of mechanical properties of conducting rubber composites based on multiwalled carbon nanotubes and Nitrile Rubber by solvent treatmentcitations
- 2017Strong Strain Sensing Performance of Natural Rubber Nanocompositescitations
- 2017Vegetable fillers for electric stimuli responsive elastomerscitations
- 2017Temperature-Dependent Reinforcement of Hydrophilic Rubber Using Ice Crystals
- 2016Improvement of actuation performance of dielectric elastomers by barium titanate and carbon black fillerscitations
- 2016Evaluation of mechanical and dynamic mechanical properties of multiwalled carbon nanotube-based ethylene–propylene copolymer composites mixed by masterbatch dilutioncitations
- 2015Rubber composites based on silane-treated stöber silica and nitrile rubber: Interaction of treated silica with rubber matrixcitations
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article
Unlocking the Potential of Lignin: Towards a Sustainable Solution for Tire Rubber Compound Reinforcement
Abstract
<p>This study tackles the persistent challenge of producing highly reinforced lignin-rubber composites, emphasizing the transformation of agro-industrial residues into value-added products. To address this challenge, we introduce a novel approach termed “in-situ surface modification utilizing a thermo-chemo-mechanical approach” which incorporates the utilization of biomass-derived kraft lignin and a thermally stable organofunctional surface modifier, specifically (3-aminopropyl) triethoxysilane. The resulting material exhibits unprecedented tensile strength (∼15 MPa) along with ∼300 % elongation at break, while typical gum rubber offers 1–2 MPa tensile strength. Additionally, for the other tensile properties like 100 %, and 200 % tensile modulus, the improvement is 7-fold (∼5.6 MPa) and 10-fold (∼11.3 MPa), respectively. Furthermore, this composite presents a higher degree of reinforcement than a passenger car radial (PCR) tire model compound (tensile strength ∼14.5 MPa, 100 % tensile modulus ∼2.2 MPa, and 200 % tensile modulus ∼5.6 MPa) comprised of silica and polysulfide-based coupling agent, with exactly a similar loading of filler. The dynamic mechanical and stress relaxation behavior of the composites are critically discussed concerning the dispersion of the lignin in the sSBR/BR rubber matrix. The morphological orientation and involved chemical interaction in the presence of a surface modifier are also studied in detail. Tear fatigue analysis using pure shear specimens indicates superior fracture toughness at a lower tearing energy regime compared to silica-filled PCR tire compounds. Overall, this study showcases the potential of lignin-reinforced elastomers, offering a promising route for sustainable engineering materials and commercial viability.</p>